Chemical Characteristics of Aerosol Composition over the Yellow Sea and the East China Sea in Autumn

作者: Hong-Hai Zhang , Gui-Peng Yang , Chun-Ying Liu , Lu-Ping Su

DOI: 10.1175/JAS-D-12-0232.1

关键词: ChemistryAerosolSulfateParticulatesChina seaAerosol compositionSea saltEnvironmental chemistryOceanography

摘要: AbstractThe total suspended particulate (TSP) samples over the Yellow Sea and East China were collected to determine major compositions of water-soluble ionic species during two cruises in autumn 2007. The aerosol exhibited an obvious regional variation between cruises, with higher concentrations (except Na+ Mg2+) northern first cruise. secondary ions [non–sea salt sulfate (nss-), , ] 11 ± 4.9, 3.1 2.1, 3.7 2.6 μg m−3, respectively, which together contributed 72% determined ion concentrations. Significant correlations these found within each sampling period, while nss-K+ nss-Ca2+ showed strong correlation other. calculated results equivalent anions (nss- ) cations ( Ca2+) that acidic mostly neutralized alkaline study areas. mass ratio nss-/ was ...

参考文章(40)
Mitsuo Uematsu, Robert A. Duce, Joseph M. Prospero, Liqi Chen, John T. Merrill, Ray L. McDonald, Transport of mineral aerosol from Asia Over the North Pacific Ocean Journal of Geophysical Research: Oceans. ,vol. 88, pp. 5343- 5352 ,(1983) , 10.1029/JC088IC09P05343
E. S. Saltzman, D. L. Savoie, J. M. Prospero, R. G. Zika, Methanesulfonic acid and non-sea-salt sulfate in pacific air: Regional and seasonal variations Journal of Atmospheric Chemistry. ,vol. 4, pp. 227- 240 ,(1986) , 10.1007/BF00052002
Ying Wang, Guoshun Zhuang, Xingying Zhang, Kan Huang, Chang Xu, Aohan Tang, Jianmin Chen, Zhisheng An, The ion chemistry;seasonal cycle;and sources of PM2.5 and TSP aerosol in Shanghai Atmospheric Environment. ,vol. 40, pp. 2935- 2952 ,(2006) , 10.1016/J.ATMOSENV.2005.12.051
Nobuo Kato, Hajime Akimoto, Anthropogenic emissions of SO2 and NOx in Asia : emission inventories Atmospheric Environment. Part A. General Topics. ,vol. 26, pp. 2997- 3017 ,(1992) , 10.1016/0960-1686(92)90291-R
Robert J. Charlson, James E. Lovelock, Meinrat O. Andreae, Stephen G. Warren, Oceanic phytoplankton, atmospheric sulphur, cloud albedo and climate Nature. ,vol. 326, pp. 655- 661 ,(1987) , 10.1038/326655A0
H MUKAI, Y YOKOUCHI, M SUZUKI, Seasonal variation of methanesulfonic acid in the atmosphere over the oki islands in the sea of ] Japan Atmospheric Environment. ,vol. 29, pp. 1637- 1648 ,(1995) , 10.1016/1352-2310(95)00057-6
David G. Streets, Carolyne Yu, Ye Wu, Mian Chin, Zongci Zhao, Tadahiro Hayasaka, Guangyu Shi, Aerosol trends over China, 1980–2000 Atmospheric Research. ,vol. 88, pp. 174- 182 ,(2008) , 10.1016/J.ATMOSRES.2007.10.016
W. Foell, C. Green, M. Amann, S. Bhattacharya, G. Carmichael, M. Chadwick, S. Cinderby, T. Haugland, J. -P. Hettelingh, L. Hordijk, J. Kuylenstierna, J. Shah, R. Shrestha, D. Streets, D. Zhao, Energy use, emissions, and air pollution reduction strategies in Asia Water Air and Soil Pollution. ,vol. 85, pp. 2277- 2282 ,(1995) , 10.1007/BF01186173
H. Akimoto, Global air quality and pollution. Science. ,vol. 302, pp. 1716- 1719 ,(2003) , 10.1126/SCIENCE.1092666
James N. Galloway, William H. Schlesinger, Hiram Levy, Anthony Michaels, Jerald L. Schnoor, Nitrogen fixation: Anthropogenic enhancement‐environmental response Global Biogeochemical Cycles. ,vol. 9, pp. 235- 252 ,(1995) , 10.1029/95GB00158