Frequency Extension to THz Range in High Pressure ESR System and Its Application to Shastry-Sutherland Model Compound SrCu$_{2}$(BO$_{3}$)$_{2}$

作者: Hitoshi Ohta , Takahiro Sakurai , Ryosuke Matsui , Kohei Kawasaki , Yuki Hirao

DOI: 10.1021/ACS.JPCB.5B03664

关键词: Excited stateHigh pressureQuantum critical pointTerahertz radiationRange (particle radiation)High transmissionMaterials scienceCeramicEnergy (signal processing)Condensed matter physics

摘要: We have made a survey of ceramics for the inner parts transmission-type pressure cell to achieve high and transmission in THz range. By using optimal combination ZrO$_{2}$-based ceramic Al$_{2}$O$_{3}$ ceramic, we succeeded obtaining up 1.5 GPa frequency region 700 GHz simultaneously. show high-pressure ESR results Shastry-Sutherland compound SrCu$_{2}$(BO$_{3}$)$_{2}$ as an application. observed direct transition modes between singlet ground state triplet excited states 1.51 successfully, obtained precise dependence gap energy. The energy is directly proved be suppressed by pressure. Moreover, found that system approaches quantum critical point with comparing data theory. This result also shows usefulness measurement study spin systems.

参考文章(31)
Zheng Weihong, C. J. Hamer, J. Oitmaa, Series expansions for a Heisenberg antiferromagnetic model for SrCu 2 (BO 3 ) 2 Physical Review B. ,vol. 60, pp. 6608- 6616 ,(1999) , 10.1103/PHYSREVB.60.6608
T. Sakurai, A. Taketani, S. Kimura, M. Yoshida, S. Okubo, H. Ohta, H. Tanaka, Y. Uwatoko, ESR Measurements of KCuCl3 under Multi Extreme Conditions LOW TEMPERATURE PHYSICS: 24th International Conference on Low Temperature Physics - LT24. ,vol. 850, pp. 1057- 1058 ,(2006) , 10.1063/1.2355067
Akihisa Koga, Norio Kawakami, Quantum Phase Transitions in the Shastry-Sutherland Model for SrCu 2 \(BO 3 \) 2 Physical Review Letters. ,vol. 84, pp. 4461- 4464 ,(2000) , 10.1103/PHYSREVLETT.84.4461
M Saruhashi, T Sakurai, T Hirano, H Ohta, S Okubo, Y Inagaki, Y Uwatoko, High-field ESR measurements of quantum spin system under high pressure Physica B-condensed Matter. ,vol. 329, pp. 963- 964 ,(2003) , 10.1016/S0921-4526(02)02624-8
T. Sakurai, M. Saruhashi, Y. Inagaki, S. Okubo, H. Ohta, H. Tanaka, Y. Uwatoko, High-field ESR measurements of CsCuCl3 under pressure Physica B-condensed Matter. ,vol. 346, pp. 221- 225 ,(2004) , 10.1016/J.PHYSB.2004.01.054
Hitoshi Ohta, Takahiro Sakurai, Masafumi Kodama, Motoi Kimata, Susumu Okubo, Makoto Yoshida, Yuko Hosokoshi, Hidekazu Tanaka, Yoshiya Uwatoko, High Field ESR Study of the Spin Gap System with the Field-Induced Phase Progress of Theoretical Physics Supplement. ,vol. 159, pp. 184- 188 ,(2005) , 10.1143/PTPS.159.184
Kohdai Fujimoto, Takahiro Sakurai, Susumu Okubo, Hitoshi Ohta, Kazuyuki Matsubayashi, Yoshiya Uwatoko, Kazutaka Kudo, Yoji Koike, Development of Hybrid-Type Pressure Cell for High-Pressure and High-Field ESR Measurement Applied Magnetic Resonance. ,vol. 44, pp. 893- 898 ,(2013) , 10.1007/S00723-013-0441-2
H. Ohta, E. Ohmichi, S. Okubo, T. Sakurai, M. Fujisawa, Development of Multi-extreme ESR Measurement System in Kobe Journal of Low Temperature Physics. ,vol. 159, pp. 302- 306 ,(2010) , 10.1007/S10909-009-0127-1
Shin Miyahara, Kazuo Ueda, Exact Dimer Ground State of the Two Dimensional Heisenberg Spin System SrCu 2 ( BO 3 ) 2 Physical Review Letters. ,vol. 82, pp. 3701- 3704 ,(1999) , 10.1103/PHYSREVLETT.82.3701
T. Sakurai, K. Fujimoto, R. Goto, S. Okubo, H. Ohta, Y. Uwatoko, Development of high-pressure and high-field ESR system using SQUID magnetometer Journal of Magnetic Resonance. ,vol. 223, pp. 41- 45 ,(2012) , 10.1016/J.JMR.2012.07.020