Superradiance and motional narrowing of exciton-polaritons in J-aggregate thin films

作者: M. Scott Bradley , Jonathan R. Tischler , Yasuhiro Shirasaki , Vladimir Bulovic

DOI: 10.1109/QELS.2007.4431481

关键词: OptoelectronicsSuperradianceThin filmExciton-polaritonsMaterials scienceMotional narrowingSpontaneous emissionExcitonPolaritonCondensed matter physicsDispersion (optics)

摘要: We investigate dispersion of J-aggregate thin films varying thickness. Reflectance measurements and simulations suggest a "superradiance" effect in thick similar to that observed multiple-quantum wells addition evidence motional narrowing.

参考文章(19)
D. G. Lidzey, D. D. C. Bradley, M. S. Skolnick, T. Virgili, S. Walker, D. M. Whittaker, Strong exciton–photon coupling in an organic semiconductor microcavity Nature. ,vol. 395, pp. 53- 55 ,(1998) , 10.1038/25692
M. S. Bradley, J. R. Tischler, V. Bulović, Layer‐by‐Layer J‐Aggregate Thin Films with a Peak Absorption Constant of 106 cm–1 Advanced Materials. ,vol. 17, pp. 1881- 1886 ,(2005) , 10.1002/ADMA.200500233
V.M. Agranovich, O.A. Dubovsky, K.I. Grigorishin, T.A. Leskova, Th. Neidlinger, P. Reineker, Superradiance of 2D Frenkel exciton-polaritons: mixing of molecular configurations and resonance interaction with the substrate principles and practice of constraint programming. ,vol. 203, pp. 11- 21 ,(1996) , 10.1016/0301-0104(96)88026-8
C. Weisbuch, M. Nishioka, A. Ishikawa, Y. Arakawa, Observation of the coupled exciton-photon mode splitting in a semiconductor quantum microcavity. Physical Review Letters. ,vol. 69, pp. 3314- 3317 ,(1992) , 10.1103/PHYSREVLETT.69.3314
R. Houdré, Early stages of continuous wave experiments on cavity-polaritons physica status solidi (b). ,vol. 242, pp. 2167- 2196 ,(2005) , 10.1002/PSSB.200560966
V. M. Agranovich, D. M. Basko, O. A. Dubovsky, Superradiance of polaritons: Crossover from two-dimensional to three-dimensional crystals Journal of Chemical Physics. ,vol. 106, pp. 3896- 3907 ,(1997) , 10.1063/1.473104
Hiroshi Fukumoto, Yoshiro Yonezawa, Layer-by-layer self-assembly of polyelectrolyte and water soluble cyanine dye Thin Solid Films. ,vol. 327, pp. 748- 751 ,(1998) , 10.1016/S0040-6090(98)00779-2
Jonathan R. Tischler, M. Scott Bradley, Vladimir Bulović, Critically coupled resonators in vertical geometry using a planar mirror and a 5 nm thick absorbing film Optics Letters. ,vol. 31, pp. 2045- 2047 ,(2006) , 10.1364/OL.31.002045
Jonathan R. Tischler, M. Scott Bradley, Vladimir Bulović, Jung Hoon Song, Arto Nurmikko, Strong coupling in a microcavity LED. Physical Review Letters. ,vol. 95, pp. 036401- ,(2005) , 10.1103/PHYSREVLETT.95.036401