Iron Isotope Effect and Local Lattice Dynamics in the (Ba, K)Fe2As2 Superconductor Studied by Temperature-Dependent EXAFS

作者: Wangsheng Chu , Jie Cheng , Shengqi Chu , Tiandou Hu , Augusto Marcelli

DOI: 10.1038/SREP01750

关键词: IsotopeExtended X-ray absorption fine structureChemical physicsPhononKinetic isotope effectLattice (order)Lattice dynamicsSuperconductivityMaterials scienceElectrical resistivity and conductivity

摘要: Currently available investigations of the isotope effect in Fe-based superconductors are all based on macroscopic resistivity and susceptibility measurements results highly controversial. Here we present an investigation Fe (Ba, K)Fe2As2 superconductor by temperature-dependent EXAFS framework Einstein model. This method separates static structural contribution local lattice contribution. Results point out substitution has a negligible inter-atomic distances. On contrary, both vibrations Fe-As Fe-Fe bonds show strong iron dependence, which is marker “intrinsic” effect. bulk to dynamics suggests phonons play important role three-dimensional electron-phonon interaction should be considered understand superconducting mechanism iron-based superconductors.

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