How to most effectively expand the global surface ozone observing network

作者: E. D. Sofen , D. Bowdalo , M. J. Evans

DOI: 10.5194/ACP-16-1445-2016

关键词: Data collectionBiomeAtmospheric chemistryAtmosphereSurface ozoneOzoneAir quality indexClimatologyEnvironmental scienceTropics

摘要: Abstract. Surface ozone observations with modern instrumentation have been made around the world for more than 40 years. Some of these as one-off activities short-term, specific science objectives and some part wider networks which provided a foundational infrastructure data collection, calibration, quality control, dissemination. These provide fundamental underpinning to our understanding tropospheric chemistry, air policy, atmosphere–biosphere interactions, etc. brought together eight single set surface observations. We investigate how representative this combined is global using output from atmospheric chemistry model. estimate that on an area basis, 25 % globe observed (34 % land, 21 % ocean). Whereas Europe North America almost complete coverage, other continents, Africa, South America, Australia, Asia (12–17 %) show significant gaps. Antarctica surprisingly well (78 %). Little monitoring occurs over oceans, tropical southern oceans particularly poorly represented. The key biomes such forests savanna completely unmonitored. A chemical cluster analysis suggests number are polluted masses, but cleaner masses whether land or ocean (especially again in tropics) significantly under-observed. current network unlikely see impact El Nino–Southern Oscillation (ENSO) may be capable detecting planetary-scale signals. Model assessment validation hampered by lack regions where models differ substantially, ability monitor likely changes next century. Using methodology we able suggest new sites would help close gap measure ozone. An additional 20 (a 20 % increase World Meteorological Organization Global Atmosphere Watch (WMO GAW) 1 % total background network) located 10 islands continental double observed. cost addition small compared expenditure composition research long-term benefit atmosphere, information will also available consideration control managers policy makers.

参考文章(32)
David M. Olson, Eric Dinerstein, The Global 200: Priority ecoregions for global conservation Annals of the Missouri Botanical Garden. ,vol. 89, pp. 199- 224 ,(2002) , 10.2307/3298564
F. Wang, A. Saiz-Lopez, A. S. Mahajan, J. C. Gómez Martín, D. Armstrong, M. Lemes, T. Hay, C. Prados-Roman, Enhanced production of oxidised mercury over the tropical Pacific Ocean: a key missing oxidation pathway Atmospheric Chemistry and Physics. ,vol. 14, pp. 1323- 1335 ,(2014) , 10.5194/ACP-14-1323-2014
Jiankai Zhang, Wenshou Tian, Ziwei Wang, Fei Xie, Feiyang Wang, The Influence of ENSO on Northern Midlatitude Ozone during the Winter to Spring Transition Journal of Climate. ,vol. 28, pp. 4774- 4793 ,(2015) , 10.1175/JCLI-D-14-00615.1
J. R. Ziemke, A. R. Douglass, L. D. Oman, S. E. Strahan, B. N. Duncan, Tropospheric ozone variability in the tropics from ENSO to MJO and shorter timescales Atmospheric Chemistry and Physics. ,vol. 15, pp. 8037- 8049 ,(2015) , 10.5194/ACP-15-8037-2015
S. Sitch, P. M. Cox, W. J. Collins, C. Huntingford, Indirect radiative forcing of climate change through ozone effects on the land-carbon sink Nature. ,vol. 448, pp. 791- 794 ,(2007) , 10.1038/NATURE06059
David W. J. Thompson, John M. Wallace, The Arctic oscillation signature in the wintertime geopotential height and temperature fields Geophysical Research Letters. ,vol. 25, pp. 1297- 1300 ,(1998) , 10.1029/98GL00950
William F. McDonnell, Keith E. Muller, Philip A. Bromberg, Carl M. Shy, Predictors of Individual Differences in Acute Response to Ozone Exposure The American review of respiratory disease. ,vol. 147, pp. 818- 825 ,(1993) , 10.1164/AJRCCM/147.4.818
Alain Marenco, Hervé Gouget, Philippe Nédélec, Jean-Pierre Pagés, Fernand Karcher, Evidence of a long-term increase in tropospheric ozone from Pic du Midi data series: Consequences: Positive radiative forcing Journal of Geophysical Research. ,vol. 99, pp. 16617- 16632 ,(1994) , 10.1029/94JD00021
Owen R Cooper, DD Parrish, Jerry Ziemke, NV Balashov, M Cupeiro, IE Galbally, S Gilge, L Horowitz, NR Jensen, J-F Lamarque, Vaishali Naik, SJ Oltmans, J Schwab, DT Shindell, Anne M Thompson, V Thouret, Y Wang, RM Zbinden, None, Global Distribution and Trends of Tropospheric Ozone: An Observation-Based Review Elementa: Science of the Anthropocene. ,vol. 2, pp. 000029- ,(2014) , 10.12952/JOURNAL.ELEMENTA.000029