The synergistic effects of dissolved oxygen and pH on N2O production in biological domestic wastewater treatment under nitrifying conditions.

作者: Pengzhang Li , Shuying Wang , Yongzhen Peng , Yue Liu , Janzhong He

DOI: 10.1080/09593330.2014.1002862

关键词: NitrificationNitrous oxideWastewaterNitrous acidChemistryAmmoniaEnvironmental chemistryPH reductionDenitrificationDenitrifying bacteria

摘要: Nitrous oxide (N2O) is a potent greenhouse gas, which produced during nitrifying and denitrifying processes. Some factors mechanisms affecting N2O emission have been reported in previous literature, but wastewater biological nitrification accompanied by dynamic process of dissolved oxygen (DO) consumption pH reduction, it more meaningful to study the synergistic effects between DO on production. In this study, production were investigated with real domestic wastewater. The results showed that high levels could improve oxidation ratio while effectively reducing accumulation N2O. was prerequisite for nitrifier denitrification; when oxidized completely, there would be no an even higher concentration factor shown directly affect emission, although free ammonia nitrous acid changed had correlati...

参考文章(37)
Alan B. Hooper, Todd Vannelli, David J. Bergmann, David M. Arciero, Enzymology of the oxidation of ammonia to nitrite by bacteria. Antonie Van Leeuwenhoek International Journal of General and Molecular Microbiology. ,vol. 71, pp. 59- 67 ,(1997) , 10.1023/A:1000133919203
K. Hanaki, Z. Hong, T. Matsuo, Production of Nitrous Oxide Gas during Denitrification of Wastewater Water Science and Technology. ,vol. 26, pp. 1027- 1036 ,(1992) , 10.2166/WST.1992.0544
Thomas F Stocker, Dahe Qin, G-K Plattner, Melinda MB Tignor, Simon K Allen, Judith Boschung, Alexander Nauels, Yu Xia, Vincent Bex, Pauline M Midgley, Climate change 2007 : the physical science basis : contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change Published in <b>2007</b> in Cambridge by Cambridge university press. ,(2007) , 10.1017/CBO9781107415324
Lisa Y. Stein, Surveying N2O-producing pathways in bacteria. Methods in Enzymology. ,vol. 486, pp. 131- 152 ,(2011) , 10.1016/B978-0-12-381294-0.00006-7
Isamu Suzuki, Usha Dular, S. C. Kwok, Ammonia or Ammonium Ion as Substrate for Oxidation by Nitrosomonas europaea Cells and Extracts Journal of Bacteriology. ,vol. 120, pp. 556- 558 ,(1974) , 10.1128/JB.120.1.556-558.1974
Raymond C. Loehr, A. C. Anthonisen, E. G. Srinath, T. B. S. Prakasam, Inhibition of nitrification by ammonia and nitrous acid. Journal of Water Pollution Control Federation. ,vol. 48, pp. 835- 852 ,(1976)
G. A. F. Ritchie, D. J. D. Nicholas, Identification of the sources of nitrous oxide produced by oxidative and reductive processes in Nitrosomonas europaea. Biochemical Journal. ,vol. 126, pp. 1181- 1191 ,(1972) , 10.1042/BJ1261181
Wenlin Jia, Shuang Liang, Jian Zhang, Huu Hao Ngo, Wenshan Guo, Yujie Yan, Yina Zou, Nitrous oxide emission in low-oxygen simultaneous nitrification and denitrification process: sources and mechanisms. Bioresource Technology. ,vol. 136, pp. 444- 451 ,(2013) , 10.1016/J.BIORTECH.2013.02.117
Pascal Wunderlin, Joachim Mohn, Adriano Joss, Lukas Emmenegger, Hansruedi Siegrist, Mechanisms of N2O production in biological wastewater treatment under nitrifying and denitrifying conditions. Water Research. ,vol. 46, pp. 1027- 1037 ,(2012) , 10.1016/J.WATRES.2011.11.080