Pr0.7Ca0.15Ba0.15MnO3 manganite: Electron paramagnetic resonance, conductivity and susceptibility

作者: A. N. Ulyanov , H. D. Quang , N. E. Pismenova , S. C. Yu , G. G. Levchenko

DOI: 10.1016/J.SSC.2012.05.024

关键词: ManganiteCurie temperatureFerromagnetismPolaronMaterials scienceElectrical resistivity and conductivityAtmospheric temperature rangeCondensed matter physicsElectron paramagnetic resonanceMagnetic susceptibility

摘要: Abstract We present a systematic experimental study of single phase Pr 0.7 Ca 0.15 Ba MnO 3 manganites. Ferromagnetic insulating state is observed in wide temperature range between the Curie point and peak resistivity temperature. Two approaches for analysis electron paramagnetic resonance (EPR) line-width (Δ H ) were considered details. The first approach based on proportionality dependencies inverse Δ . second model where ∝1/ Tχ dc ( χ static magnetic susceptibility). For studied manganites resistivity, associated with grain boundary scattering, follows Mott law; EPR line-width, suggested to be an intrinsic property, well described polaron hopping model.

参考文章(32)
A. K. Heilman, Y. Y. Xue, B. Lorenz, B. J. Campbell, J. Cmaidalka, R. L. Meng, Y. S. Wang, C. W. Chu, Distinct insulating state below the Curie point in Pr 0.7 Ba 0.3 MnO 3 Physical Review B. ,vol. 65, pp. 2144231- 2144235 ,(2002) , 10.1103/PHYSREVB.65.214423
D. L. Huber, G. Alejandro, A. Caneiro, M. T. Causa, F. Prado, M. Tovar, S. B. Oseroff, EPR linewidths in La 1-x Ca x MnO 3 : 0<=x<=1 Physical Review B. ,vol. 60, pp. 12155- 12161 ,(1999) , 10.1103/PHYSREVB.60.12155
A. Shengelaya, Guo-meng Zhao, H. Keller, K. A. Müller, B. I. Kochelaev, EPR inLa1−xCaxMnO3: Relaxation and bottleneck Physical Review B. ,vol. 61, pp. 5888- 5890 ,(2000) , 10.1103/PHYSREVB.61.5888
H. Nojiri, K. Kaneko, M. Motokawa, K. Hirota, Y. Endoh, K. Takahashi, Two ferromagnetic phases in La 1-x Sr x MnO 3 (x~1/8) Physical Review B. ,vol. 60, pp. 4142- 4148 ,(1999) , 10.1103/PHYSREVB.60.4142
A. N. Ulyanov, S. C. Yu, N. Yu. Starostyuk, N. E. Pismenova, Y. M. Moon, K. W. Lee, Phase diagram and anomalous properties of La[sub 0.7]M[sub 0.3]MnO[sub 3] lanthanum manganites near the structural phase transition Journal of Applied Physics. ,vol. 91, pp. 8900- 8902 ,(2002) , 10.1063/1.1446132
D.L. Huber, D. Laura-Ccahuana, M. Tovar, M.T. Causa, Electron spin resonance linewidth, susceptibility, and conductivity in doped manganites Journal of Magnetism and Magnetic Materials. ,vol. 310, ,(2007) , 10.1016/J.JMMM.2006.10.715
A.N. Ulyanov, Hoang Duc Quang, N.E. Pismenova, Seong-Cho Yu, EPR and resistivity study of Pr/sub 0.7/Ba/sub 0.3/MnO/sub 3/ manganite IEEE Transactions on Magnetics. ,vol. 41, pp. 2745- 2747 ,(2005) , 10.1109/TMAG.2005.854828
D. L. Lyfar, S. M. Ryabchenko, V. N. Krivoruchko, S. I. Khartsev, A. M. Grishin, Microwave absorption in a thinLa0.7Sr0.3MnO3film: Manifestation of colossal magnetoresistance Physical Review B. ,vol. 69, pp. 100409- ,(2004) , 10.1103/PHYSREVB.69.100409
B. F. Woodfield, M. L. Wilson, J. M. Byers, Low-Temperature Specific Heat of La{sub 1-x}Sr{sub x}MnO{sub 3+{delta}} Physical Review Letters. ,vol. 78, pp. 3201- 3204 ,(1997) , 10.1103/PHYSREVLETT.78.3201
V. A. Atsarkin, V. V. Demidov, G. A. Vasneva, K. Conder, Critical slowing down of longitudinal spin relaxation in La 1-x Ca x MnO 3 Physical Review B. ,vol. 63, pp. 092405- ,(2001) , 10.1103/PHYSREVB.63.092405