Fast operando spectroscopy tracking in situ generation of rich defects in silver nanocrystals for highly selective electrochemical CO2 reduction.
作者： Zhiwei Hu , Zongping Shao , Zongping Shao , Jie Dai , Daqin Guan
DOI: 10.1038/S41467-021-20960-8
关键词: Electrochemistry 、 Materials science 、 Faraday efficiency 、 Catalysis 、 Absorption spectroscopy 、 Electrochemical reduction of carbon dioxide 、 Reversible hydrogen electrode 、 Overpotential 、 Operando spectroscopy 、 Chemical engineering
摘要: … DFT calculations demonstrated that the adsorption of intermediate COOH is strengthened on Ag atoms surrounding the defect sites, benefiting the activation of CO 2 . Therefore, …
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