Non-Markovian effects of intermolecular vibrational coherence on femtosecond time-resolved coherent anti-Stokes Raman scattering from molecules in condensed phases
作者： M. Sugawara , M. Hayashi , Y. Fujimura
DOI: 10.1016/0009-2614(92)85213-T
关键词: Raman scattering 、 Analytical chemistry 、 Quantum beats 、 Molecule 、 Coherent anti-Stokes Raman spectroscopy 、 Femtosecond 、 Molecular physics 、 Coherence (physics) 、 Intermolecular force 、 Markov process 、 Chemistry
摘要: Abstract Non-Markovian effects of intermolecular vibrational coherences on femtosecond time-resolved coherent anti-Stokes Raman scattering (CARS) from a molecular mixture are theoretically studied. The non-Markovian behavior coherence transfers based stochastic model results in the suppresion frequency shifts quantum beats CARS profiles compared with case Markovian approximation.
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