Satellite observations cap the atmospheric organic aerosol budget
作者： Colette L. Heald , David A. Ridley , Sonia M. Kreidenweis , Easan E. Drury
DOI: 10.1029/2010GL045095
关键词: Atmospheric sciences 、 Satellite 、 Environmental science 、 Soot 、 Atmosphere 、 Geos chem 、 Earth's energy budget 、 Aerosol
摘要: [1] Limited understanding of the production and loss organic aerosol (OA) to atmosphere has resulted in poorly constrained source estimates ranging from 140 910 TgCyr−1 [Goldstein Galbally, 2007]. We use satellite observations quantitatively estimate atmospheric burden associated production. find that attributing mid-visible continental optical depth (AOD) observed by MISR entirely OA implies a global 430 sub-micron OA. model (GEOS-Chem) remove contribution inorganic aerosol, dust soot AOD derive 150 (equivalent 2.5 TgC), with 80% uncertainty. This result significantly reduces uncertainty budget provides an upper limit for “missing source”
harvard.edu
agu.org参考文章(37)
Q. Zhang, J. L. Jimenez, M. R. Canagaratna, J. D. Allan, H. Coe, I. Ulbrich, M. R. Alfarra, A. Takami, A. M. Middlebrook, Y. L. Sun, K. Dzepina, E. Dunlea, K. Docherty, P. F. DeCarlo, D. Salcedo, T. Onasch, J. T. Jayne, T. Miyoshi, A. Shimono, S. Hatakeyama, N. Takegawa, Y. Kondo, J. Schneider, F. Drewnick, S. Borrmann, S. Weimer, K. Demerjian, P. Williams, K. Bower, R. Bahreini, L. Cottrell, R. J. Griffin, J. Rautiainen, J. Y. Sun, Y. M. Zhang, D. R. Worsnop, Ubiquity and dominance of oxygenated species in organic aerosols in anthropogenically-influenced Northern Hemisphere midlatitudes Geophysical Research Letters. ,vol. 34, ,(2007) , 10.1029/2007GL029979
Intergovernmental Panel on Climate Change, Climate Change 2007 Barker, Terry; Bashmakov, Igor; Alharthi, Awwad; Ammann, Markus; Cifuentes, Luis; Drexhage, John; Maosheng, Duan; Edenhofer, Ottmar; Flannery, Brian; Grubb, Michael; Hoogwijk, Monique; Ibitoye, Francis; Jepma, Catrinus; Pizer, William; Yamaji, Kenji; Awerbuch, Shimon; Bernstein, Lenny; Faaij, Andre; Hayami, Hitoshi; Heggedal, Tom; Kverndokk, Snorre; Latham, John; Michaelowa, Axel; Popp, David; Read, Peter; Schleicher, Stefan; Smith, Mike; Toth, Ferenc (2007). Mitigation from a cross-sectoral perspectiv. In: Metz, Bert; Davidson, Ogunlade; Bosch, Peter; Dave, Rutu; Meyer, Leo. Climate change 2007: mitigation of climate change. Cambridge: Cambridge University Press, 619-690.. pp. 619- 690 ,(2007) , 10.1017/CBO9780511546013
H. Pitcher, J. Alcamo, H.-H. Rogner, A. Grübler, N. Nakicenovic, K. Riahi, Tae Yong Jung, Jørgen Villy Fenhann, W. Pepper, M. Schlesinger, S. Smith, T. Kram, T. Morita, L. Price, A. Sankovski, R. Swart, L. Michaelis, G. Davis, S. Mori, N. Victor, P. Shukla, Z. Dadi, A. Roehrl, S. Gaffin, E. L. La Rovere, B. de Vries, S. van Rooijen, K. Gregory, Special report on emissions scenarios : a special report of Working group III of the Intergovernmental Panel on Climate Change Cambridge University Press. ,(2000)
Rokjin J Park, Daniel J Jacob, Brendan D Field, Robert M Yantosca, Mian Chin, Natural and transboundary pollution influences on sulfate-nitrate-ammonium aerosols in the United States: Implications for policy Journal of Geophysical Research. ,vol. 109, ,(2004) , 10.1029/2003JD004473
E. J. Dunlea, P. F. DeCarlo, A. C. Aiken, J. R. Kimmel, R. E. Peltier, R. J. Weber, J. Tomlinson, D. R. Collins, Y. Shinozuka, C. S. McNaughton, S. G. Howell, A. D. Clarke, L. K. Emmons, E. C. Apel, G. G. Pfister, A. van Donkelaar, R. V. Martin, D. B. Millet, C. L. Heald, J. L. Jimenez, Evolution of Asian aerosols during transpacific transport in INTEX-B Atmospheric Chemistry and Physics. ,vol. 9, pp. 7257- 7287 ,(2009) , 10.5194/ACP-9-7257-2009
E Dinar, A Abo Riziq, C Spindler, C Erlick, G Kiss, Yinon Rudich, None, The complex refractive index of atmospheric and model humic-like substances (HULIS) retrieved by a cavity ring down aerosol spectrometer (CRD-AS) Faraday Discussions. ,vol. 137, pp. 279- 295 ,(2008) , 10.1039/B703111D
Q. Chen, D. K. Farmer, J. Schneider, S. R. Zorn, C. L. Heald, T. G. Karl, A. Guenther, J. D. Allan, N. Robinson, H. Coe, J. R. Kimmel, T. Pauliquevis, S. Borrmann, U. Pöschl, M. O. Andreae, P. Artaxo, J. L. Jimenez, S. T. Martin, Mass spectral characterization of submicron biogenic organic particles in the Amazon Basin Geophysical Research Letters. ,vol. 36, ,(2009) , 10.1029/2009GL039880
Colette L. Heald, Daniel J. Jacob, Solène Turquety, Rynda C. Hudman, Rodney J. Weber, Amy P. Sullivan, Richard E. Peltier, Eliot L. Atlas, Joost A. de Gouw, Carsten Warneke, John S. Holloway, J. Andrew Neuman, Frank M. Flocke, John H. Seinfeld, Concentrations and sources of organic carbon aerosols in the free troposphere over North America Journal of Geophysical Research. ,vol. 111, ,(2006) , 10.1029/2006JD007705
Rainer Volkamer, Jose L. Jimenez, Federico San Martini, Katja Dzepina, Qi Zhang, Dara Salcedo, Luisa T. Molina, Douglas R. Worsnop, Mario J. Molina, Secondary organic aerosol formation from anthropogenic air pollution: Rapid and higher than expected Geophysical Research Letters. ,vol. 33, ,(2006) , 10.1029/2006GL026899
Randall V. Martin, Daniel J. Jacob, Robert M. Yantosca, Mian Chin, Paul Ginoux, Global and regional decreases in tropospheric oxidants from photochemical effects of aerosols Journal of Geophysical Research. ,vol. 108, pp. 4097- ,(2003) , 10.1029/2002JD002622