Removal of trace organic chemicals in onsite wastewater soil treatment units: a laboratory experiment.

作者: Jennifer Teerlink , Virtudes Martínez-Hernández , Christopher P. Higgins , Jörg E. Drewes

DOI: 10.1016/J.WATRES.2012.06.024

关键词: EffluentSurface waterEnvironmental chemistryGroundwaterNitrateWastewaterWater qualityOnsite sewage facilityChemistryDissolved organic carbon

摘要: Onsite wastewater treatment is used by 20% of residences in the United States. The ability these systems, specifically soil units (STUs), to attenuate trace organic chemicals (TOrCs) not well understood. TOrCs released STUs pose a potential risk downstream groundwater and hydraulically-connected surface water that may be as drinking source. A series bench-scale experiments were conducted using sand columns represent evaluate efficacy TOrC attenuation function hydraulic loading rate (1, 4, 8, 12, 30 cm/day). Each was examined triplicate experimental columns. Columns initially seeded with raw establish microbial community, after which they fed synthetic spiked 17 TOrCs, four equal doses per day, provide consistent influent quality. After an initial start-up phase, effluent from all consistently demonstrated >90% reductions dissolved carbon nearly complete (>85%) oxidation ammonia nitrate, comparable performance field STUs. results this study suggest are capable attenuating many present domestic wastewater, but compound-specific. subset exhibited inverse relationship efficiency. Atenolol, cimetidine, TCPP more effectively attenuated over time each experiment, suggesting community evolved stage where biotransformed. Aerobic conditions compared anaerobic resulted efficient acetaminophen cimetidine.

参考文章(43)
Donald Langmuir, Aqueous Environmental Geochemistry ,(1997)
N. Moelants, G. Janssen, I. Smets, J. Van Impe, Field performance assessment of onsite individual wastewater treatment systems. Water Science and Technology. ,vol. 58, pp. 1- 6 ,(2008) , 10.2166/WST.2008.325
L.A. Schipper, S.C. Cameron, S. Warneke, Nitrate removal from three different effluents using large-scale denitrification beds Ecological Engineering. ,vol. 36, pp. 1552- 1557 ,(2010) , 10.1016/J.ECOLENG.2010.02.007
Alan M. Vajda, Larry B. Barber, James L. Gray, Elena M. Lopez, John D. Woodling, David O. Norris, Reproductive disruption in fish downstream from an estrogenic wastewater effluent. Environmental Science & Technology. ,vol. 42, pp. 3407- 3414 ,(2008) , 10.1021/ES0720661
Amy L. Filby, Eduarda M. Santos, Karen L. Thorpe, Gerd Maack, Charles R. Tyler, Gene Expression Profiling for Understanding Chemical Causation of Biological Effects for Complex Mixtures: A Case Study on Estrogens Environmental Science & Technology. ,vol. 41, pp. 8187- 8194 ,(2007) , 10.1021/ES071278V
James W. McKinley, Robert L. Siegrist, Accumulation of Organic Matter Components in Soil under Conditions Imposed by Wastewater Infiltration Soil Science Society of America Journal. ,vol. 74, pp. 1690- 1700 ,(2010) , 10.2136/SSSAJ2009.0395
I.M. Verstraeten, G.S. Fetterman, M.T. Meyer, T. Bullen, S.K. Sebree, Use of tracers and isotopes to evaluate vulnerability of water in domestic wells to septic waste Ground Water Monitoring and Remediation. ,vol. 25, pp. 107- 117 ,(2005) , 10.1111/J.1745-6592.2005.0015.X
Niina M. Vieno, Heli Härkki, Tuula Tuhkanen, Leif Kronberg, Occurrence of pharmaceuticals in river water and their elimination in a pilot-scale drinking water treatment plant. Environmental Science & Technology. ,vol. 41, pp. 5077- 5084 ,(2007) , 10.1021/ES062720X
Pierre Labadie, Andrew B. Cundy, Kevin Stone, Michael Andrews, Sam Valbonesi, Elizabeth M. Hill, Evidence for the Migration of Steroidal Estrogens through River Bed Sediments Environmental Science & Technology. ,vol. 41, pp. 4299- 4304 ,(2007) , 10.1021/ES063062J