Temperature-dependent properties of the magnetic order in single-crystal BiFeO 3

作者: M. Ramazanoglu , W. Ratcliff , Y. J. Choi , Seongsu Lee , S.-W. Cheong

DOI: 10.1103/PHYSREVB.83.174434

关键词: FerroelectricityMaterials scienceMagnetic domainCondensed matter physicsSingle crystalNeutron diffractionCrystallographic point groupMagnetizationAnharmonicityMultiferroics

摘要: We report neutron diffraction and magnetization studies of the magnetic order in multiferroic BiFeO${}_{3}$. In ferroelectric monodomain single crystals, there are three cycloidal domains with propagation vectors equivalent by crystallographic symmetry. The cycloid period slowly grows increasing temperature. domain populations do not change temperature except close vicinity N\'eel temperature, at which, addition, a small jump is observed. No evidence for spin-reorientation transitions proposed previous Raman dielectric found. slightly anharmonic $T=5$ K. anharmonicity much smaller than previously reported nuclear resonance studies. At room circular observed, within errors. argue that observed provides important clues understanding electromagnons

参考文章(35)
Gustau Catalan, James F. Scott, Physics and Applications of Bismuth Ferrite Advanced Materials. ,vol. 21, pp. 2463- 2485 ,(2009) , 10.1002/ADMA.200802849
Sang-Wook Cheong, Maxim Mostovoy, Multiferroics: a magnetic twist for ferroelectricity Nature Materials. ,vol. 6, pp. 13- 20 ,(2007) , 10.1038/NMAT1804
R. Ramesh, Nicola A. Spaldin, Multiferroics: progress and prospects in thin films. Nature Materials. ,vol. 6, pp. 21- 29 ,(2007) , 10.1038/NMAT1805
T Zhao, A Scholl, F Zavaliche, K Lee, M Barry, A Doran, MP Cruz, YH Chu, C Ederer, NA Spaldin, RR Das, DM Kim, SH Baek, CB Eom, Rm Ramesh, None, Electrical control of antiferromagnetic domains in multiferroic BiFeO3 films at room temperature. Nature Materials. ,vol. 5, pp. 823- 829 ,(2006) , 10.1038/NMAT1731
Seoungsu Lee, W. Ratcliff, S-W. Cheong, V. Kiryukhin, Electric field control of the magnetic state in BiFeO3 single crystals Applied Physics Letters. ,vol. 92, pp. 192906- ,(2008) , 10.1063/1.2930678
Claude Ederer, Nicola A. Spaldin, Weak ferromagnetism and magnetoelectric coupling in bismuth ferrite Physical Review B. ,vol. 71, pp. 060401- ,(2005) , 10.1103/PHYSREVB.71.060401
S. Lisenkov, D. Rahmedov, L. Bellaiche, Electric-field-induced paths in multiferroic BiFeO3 from atomistic simulations. Physical Review Letters. ,vol. 103, pp. 047204- ,(2009) , 10.1103/PHYSREVLETT.103.047204
T. Choi, S. Lee, Y. J. Choi, V. Kiryukhin, S.-W. Cheong, Switchable ferroelectric diode and photovoltaic effect in BiFeO3. Science. ,vol. 324, pp. 63- 66 ,(2009) , 10.1126/SCIENCE.1168636
Seongsu Lee, Taekjib Choi, W. Ratcliff, R. Erwin, S-W. Cheong, V. Kiryukhin, Single ferroelectric and chiral magnetic domain of single-crystalline BiFeO 3 in an electric field Physical Review B. ,vol. 78, pp. 100101- ,(2008) , 10.1103/PHYSREVB.78.100101