Persistent Infrared Spectral Hole-Burning for Impurity Vibrational Modes in Solids
作者： A. J. Sievers , W. E. Moerner
DOI: 10.1007/978-3-642-83290-1_6
关键词: Impurity 、 Perrhenate 、 Molecule 、 Molecular vibration 、 Photochemistry 、 Spectral hole burning 、 Ion 、 Infrared 、 Molecular physics 、 Chemistry 、 Halide
摘要: One unusual group of excitations in which persistent spectral hole-burning has been observed consists infrared vibrational transitions impurity molecules solids. Examples include 1,2-difluoroethane rare gas matrices, perrhenate ions alkali halide crystals, and most recently, cyanide nitrite KBr. The hole formation mechanisms involve molecular reorientation or conformational changes at low temperatures induced by excitation an internal mode the molecule.
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