Real-time measurements of IVR versus inferences from spectral broadening data: the alkylanilines “ring + tail” system
作者： J.S. Baskin , M. Dantus , A.H. Zewail
DOI: 10.1016/0009-2614(86)80242-1
关键词: Coherence (signal processing) 、 Ultraviolet radiation 、 Picosecond 、 Doppler broadening 、 Quantum 、 Chemistry 、 Time resolution 、 Optics 、 Molecular beam 、 Atomic physics 、 Physical and Theoretical Chemistry 、 General Physics and Astronomy
摘要: We report on picosecond/molecular beam studies of alkylanilines. The reveal important discrepancies between real-time measurements and inferences from spectral broadening data. observe quantum recurrences we find that the observed severe congestion does not correspond to coherence. effect mode symmetry energy IVR dynamics is also examined.
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