Kinematics and dynamics of atomic-beam scattering on liquid and self-assembled monolayer surfaces.
作者： William A. Alexander , Jianming Zhang , Vanessa J. Murray , Gilbert M. Nathanson , Timothy K. Minton
DOI: 10.1039/C2FD20034A
关键词: Scattering 、 Molecular dynamics 、 Atom 、 Effective mass (solid-state physics) 、 Argon 、 Molecule 、 Chemistry 、 Atomic physics 、 Self-assembled monolayer 、 Kinematics
摘要: We have conducted investigations of the energy transfer dynamics atomic oxygen and argon scattering from hydrocarbon fluorocarbon surfaces. In light these results, we appraise applicability value a kinematic model, which views gas-surface interaction as gas-phase-like collision between an incident atom or molecule localized region surface with effective mass. applied this model to interpret mass when atoms strike two different surfaces under identical bombardment conditions. To end, collected new data, re-examined existing data sets both molecular-beam experiments molecular simulations. seek identify trends that could lead robust general understanding processes induced by collisions gas-phase species liquid semi-solid
rsc.org
harvard.edu
sci-hub.se 参考文章(40)
Gang‐yu Liu, Paul Fenter, Christopher E. D. Chidsey, D. Frank Ogletree, Peter Eisenberger, Miquel Salmeron, AN UNEXPECTED PACKING OF FLUORINATED N-ALKANE THIOLS ON AU(111) : A COMBINED ATOMIC FORCE MICROSCOPY AND X-RAY DIFFRACTION STUDY Journal of Chemical Physics. ,vol. 101, pp. 4301- 4306 ,(1994) , 10.1063/1.467479
Tianying Yan, William L. Hase, Comparisons of Models for Simulating Energy Transfer in Ne-Atom Collisions with an Alkyl Thiolate Self-Assembled Monolayer† Journal of Physical Chemistry B. ,vol. 106, pp. 8029- 8037 ,(2002) , 10.1021/JP025902W
Saulo A. Vázquez, John R. Morris, Asif Rahaman, Oleg A. Mazyar, Grigoriy Vayner, Srirangam V. Addepalli, William L. Hase, Emilio Martínez-Núñez, Inelastic scattering dynamics of Ar from a perfluorinated self-assembled monolayer surface. Journal of Physical Chemistry A. ,vol. 111, pp. 12785- 12794 ,(2007) , 10.1021/JP076431M
B. Scott Day, John R. Morris, Packing density and structure effects on energy-transfer dynamics in argon collisions with organic monolayers. Journal of Chemical Physics. ,vol. 122, pp. 234714- 234714 ,(2005) , 10.1063/1.1924693
Diego Troya, Dynamics of collisions of hydroxyl radicals with fluorinated self-assembled monolayers Theoretical Chemistry Accounts. ,vol. 131, pp. 1072- ,(2012) , 10.1007/S00214-011-1072-Z
Jay W. Ponder, Frederic M. Richards, An efficient newton-like method for molecular mechanics energy minimization of large molecules Journal of Computational Chemistry. ,vol. 8, pp. 1016- 1024 ,(1987) , 10.1002/JCC.540080710
Gilbert M. Nathanson, Molecular beam studies of gas-liquid interfaces. Annual Review of Physical Chemistry. ,vol. 55, pp. 231- 255 ,(2004) , 10.1146/ANNUREV.PHYSCHEM.55.091602.094357
Diego Troya *, George C. Schatz †, Hyperthermal chemistry in the gas phase and on surfaces: Theoretical studies International Reviews in Physical Chemistry. ,vol. 23, pp. 341- 373 ,(2004) , 10.1080/0144235042000298484
Michael Graupe, Thomas Koini, Vincent Y Wang, George M Nassif, Ramon Colorado, Ramon J Villazana, Henry Dong, Yasuhiro F Miura, Olga E Shmakova, T.Randall Lee, Terminally perfluorinated long-chain alkanethiols Journal of Fluorine Chemistry. ,vol. 93, pp. 107- 115 ,(1999) , 10.1016/S0022-1139(98)00284-X
J. J. Nogueira, S. A. Vázquez, U. Lourderaj, W. L. Hase, E. Martínez-Núñez, Chemical Dynamics Simulations of CO2 in the Ground and First Excited Bend States Colliding with a Perfluorinated Self-Assembled Monolayer Journal of Physical Chemistry C. ,vol. 114, pp. 18455- 18464 ,(2010) , 10.1021/JP103511G