Kinetics of the uptake of SO2 on mineral oxides: Improved initial uptake coefficients at 298 K from pulsed Knudsen cell experiments
作者： Sabine Seisel , Thorsten Keil , Yu Lian , Reinhard Zellner
DOI: 10.1002/KIN.20148
关键词: Mineral dust 、 Kinetics 、 Mineral 、 Saturation (chemistry) 、 Diffusion 、 Pulsed mode 、 Knudsen cell 、 Analytical chemistry 、 Chemistry 、 Reactivity (chemistry)
摘要: … SO 2 is introduced into the Knudsen reactor from the gas-handling system and leaves the Knudsen reactor through … Important parameters of the Knudsen cell are summarized in Table I. …
sci-hub.se 参考文章(16)
Sabine Seisel, Yu Lian, Thorsten Keil, Maxim E. Trukhin, Reinhard Zellner, Kinetics of the interaction of water vapour with mineral dust and soot surfaces at T=298 K Physical Chemistry Chemical Physics. ,vol. 6, pp. 1926- 1932 ,(2004) , 10.1039/B314568A
D Jacob, Heterogeneous chemistry and tropospheric ozone Atmospheric Environment. ,vol. 34, pp. 2131- 2159 ,(2000) , 10.1016/S1352-2310(99)00462-8
D. M. Golden, G. N. Spokes, S. W. Benson, Pyrolyse bei sehr kleinem Druck (VLPP); eine vielseitige kinetische Methode Angewandte Chemie. ,vol. 85, pp. 602- 614 ,(1973) , 10.1002/ANGE.19730851403
François Caloz, Frederick F. Fenter, Kevin D. Tabor, Michel J. Rossi, Paper I: Design and construction of a Knudsen-cell reactor for the study of heterogeneous reactions over the temperature range 130–750 K: Performances and limitations Review of Scientific Instruments. ,vol. 68, pp. 3172- 3179 ,(1997) , 10.1063/1.1148263
Frederick F Fenter, François Caloz, Michel J Rossi, None, Heterogeneous Kinetics of N2O5 Uptake on Salt, with a Systematic Study of the Role of Surface Presentation (for N2O5 and HNO3) The Journal of Physical Chemistry. ,vol. 100, pp. 1008- 1019 ,(1996) , 10.1021/JP9503829
Michel J. Rossi, Heterogeneous reactions on salts. Chemical Reviews. ,vol. 103, pp. 4823- 4882 ,(2003) , 10.1021/CR020507N
Courtney R. Usher, Amy E. Michel, Vicki H. Grassian, Reactions on mineral dust. Chemical Reviews. ,vol. 103, pp. 4883- 4939 ,(2003) , 10.1021/CR020657Y
P. Li, H. A. Al-Abadleh, V. H. Grassian, Measuring Heterogeneous Uptake Coefficients of Gases on Solid Particle Surfaces with a Knudsen Cell Reactor: Complications Due to Surface Saturation and Gas Diffusion into Underlying Layers Journal of Physical Chemistry A. ,vol. 106, pp. 1210- 1219 ,(2002) , 10.1021/JP011828Q
A. L. Goodman, P. Li, C. R. Usher, V. H. Grassian, Heterogeneous Uptake of Sulfur Dioxide On Aluminum and Magnesium Oxide Particles Journal of Physical Chemistry A. ,vol. 105, pp. 6109- 6120 ,(2001) , 10.1021/JP004423Z
Rachel C. Hoffman, Michael E. Gebel, Brigitte S. Fox, Barbara J. Finlayson-Pitts, Knudsen cell studies of the reactions of N2O5 and ClONO2 with NaCl: development and application of a model for estimating available surface areas and corrected uptake coefficients Physical Chemistry Chemical Physics. ,vol. 5, pp. 1780- 1789 ,(2003) , 10.1039/B301126G