Destructive quantum interference in transport through molecules with electron-electron and electron-vibration interactions

作者: P Roura-Bas , F Güller , L Tosi , A A Aligia

DOI: 10.1088/1361-648X/AB3684

关键词: Interference (wave propagation)Molecular physicsConductanceMoleculeMolecular vibrationOrders of magnitude (time)Molecular orbitalElectronTransistorPhysics

摘要: We study the transport through a molecular junction exhibiting interference effects. show that these effects can still be observed in presence of vibrations if Coulomb repulsion is taken into account. In Kondo regime, conductance changed by several orders magnitude tuning levels molecule, or displacing contact between two atoms, from nearly perfect destructive to values order 2e 2 /h expected systems. also this large change robust for reasonable temperatures and voltages symmetric asymmetric tunnel couplings source-drain electrodes orbitals. This relevant development quantum effect transistors based on junctions.

参考文章(56)
Sriharsha V. Aradhya, Latha Venkataraman, Single-molecule junctions beyond electronic transport Nature Nanotechnology. ,vol. 8, pp. 399- 410 ,(2013) , 10.1038/NNANO.2013.91
David M. Cardamone, Charles A. Stafford, Sumit Mazumdar, Controlling Quantum Transport through a Single Molecule Nano Letters. ,vol. 6, pp. 2422- 2426 ,(2006) , 10.1021/NL0608442
San-Huang Ke, Weitao Yang, Harold U. Baranger, Quantum-interference-controlled molecular electronics. Nano Letters. ,vol. 8, pp. 3257- 3261 ,(2008) , 10.1021/NL8016175
Georg Begemann, Dana Darau, Andrea Donarini, Milena Grifoni, Symmetry fingerprints of a benzene single-electron transistor: Interplay between Coulomb interaction and orbital symmetry Physical Review B. ,vol. 77, pp. 201406- ,(2008) , 10.1103/PHYSREVB.77.201406
Andrea Donarini, Georg Begemann, Milena Grifoni, All-electric spin control in interference single electron transistors. Nano Letters. ,vol. 9, pp. 2897- 2902 ,(2009) , 10.1021/NL901199P
Julián Rincón, K. Hallberg, A. A. Aligia, S. Ramasesha, Quantum interference in coherent molecular conductance Physical Review Letters. ,vol. 103, pp. 266807- ,(2009) , 10.1103/PHYSREVLETT.103.266807
L Tosi, P Roura-Bas, A A Aligia, Nonequilibrium conductance through a benzene molecule in the Kondo regime arXiv: Mesoscale and Nanoscale Physics. ,(2012) , 10.1088/0953-8984/24/36/365301
Marc H. Garner, Haixing Li, Yan Chen, Timothy A. Su, Zhichun Shangguan, Daniel W. Paley, Taifeng Liu, Fay Ng, Hexing Li, Shengxiong Xiao, Colin Nuckolls, Latha Venkataraman, Gemma C. Solomon, Comprehensive suppression of single-molecule conductance using destructive σ-interference. Nature. ,vol. 558, pp. 415- 419 ,(2018) , 10.1038/S41586-018-0197-9
Yueqi Li, Marius Buerkle, Guangfeng Li, Ali Rostamian, Hui Wang, Zixiao Wang, David R. Bowler, Tsuyoshi Miyazaki, Limin Xiang, Yoshihiro Asai, Gang Zhou, Nongjian Tao, Gate controlling of quantum interference and direct observation of anti-resonances in single molecule charge transport Nature Materials. ,vol. 18, pp. 357- 363 ,(2019) , 10.1038/S41563-018-0280-5