Adsorption transition of a grafted ferromagnetic filament controlled by external magnetic fields.

作者: Pedro A Sánchez , Ekaterina V Novak , Elena S Pyanzina , Sofia S Kantorovich , Joan J Cerdà

DOI: 10.1103/PHYSREVE.102.022609

关键词: Field strengthMagnetic fluxChemical physicsAdsorptionFerromagnetismField (physics)Magnetic fieldProtein filamentLangevin dynamicsMaterials science

摘要: Extensive Langevin dynamics simulations are used to characterize the adsorption transition of a flexible magnetic filament grafted onto an attractive planar surface. Our results identify different structural transitions at ratios thermal energy surface attraction strength: straightening, adsorption, and flux closure. The temperature is found be higher in comparison equivalent nonmagnetic chain. has been also investigated under application static homogeneous external field. We that strength orientation field can control process, providing precise switching mechanism. Interestingly, we have observed characteristic tilt angle point related by simple power law.

参考文章(65)
Ye Tian, Tong Wang, Wenyan Liu, Huolin L. Xin, Huilin Li, Yonggang Ke, William M. Shih, Oleg Gang, Prescribed nanoparticle cluster architectures and low-dimensional arrays built using octahedral DNA origami frames Nature Nanotechnology. ,vol. 10, pp. 637- 644 ,(2015) , 10.1038/NNANO.2015.105
John D. Weeks, David Chandler, Hans C. Andersen, Role of Repulsive Forces in Determining the Equilibrium Structure of Simple Liquids The Journal of Chemical Physics. ,vol. 54, pp. 5237- 5247 ,(1971) , 10.1063/1.1674820
Pedro A Sánchez, Elena S Pyanzina, Ekaterina V Novak, Joan J Cerdà, Tomàs Sintes, Sofia S Kantorovich, None, Magnetic filament brushes: tuning the properties of a magnetoresponsive supracolloidal coating. Faraday Discussions. ,vol. 186, pp. 241- 263 ,(2016) , 10.1039/C5FD00133A
Dean S. Wood, Philip J. Camp, Modeling the properties of ferrogels in uniform magnetic fields Physical Review E. ,vol. 83, pp. 011402- ,(2011) , 10.1103/PHYSREVE.83.011402
Serena A. Corr, Stephen J. Byrne, Renata Tekoriute, Carla J. Meledandri, Dermot F. Brougham, Marina Lynch, Christian Kerskens, Laurence O'Dwyer, Yurii K. Gun'ko, Linear assemblies of magnetic nanoparticles as MRI contrast agents. Journal of the American Chemical Society. ,vol. 130, pp. 4214- 4215 ,(2008) , 10.1021/JA710172Z
Jason J. Benkoski, Steven E. Bowles, Bryan D. Korth, Ronald L. Jones, Jack F. Douglas, Alamgir Karim, Jeffrey Pyun, Field induced formation of mesoscopic polymer chains from functional ferromagnetic colloids. Journal of the American Chemical Society. ,vol. 129, pp. 6291- 6297 ,(2007) , 10.1021/JA070779D
Mitsusuke Tarama, Peet Cremer, Dmitry Y. Borin, Stefan Odenbach, Hartmut Löwen, Andreas M. Menzel, Tunable dynamic response of magnetic gels: impact of structural properties and magnetic fields. Physical Review E. ,vol. 90, pp. 042311- ,(2014) , 10.1103/PHYSREVE.90.042311
T. Sintes, K. Sumithra, E. Straube, Adsorption of semiflexible polymers on flat, homogeneous surfaces Macromolecules. ,vol. 34, pp. 1352- 1357 ,(2001) , 10.1021/MA000493S
Leilei Sun, Yongmei Zheng, Bio-inspired artificial cilia with magnetic dynamic properties Frontiers of Materials Science. ,vol. 9, pp. 178- 184 ,(2015) , 10.1007/S11706-015-0291-Y
A. C. Balazs, T. Emrick, T. P. Russell, Nanoparticle Polymer Composites: Where Two Small Worlds Meet Science. ,vol. 314, pp. 1107- 1110 ,(2006) , 10.1126/SCIENCE.1130557