Fe-Doped TiO2 Supported on HY Zeolite for Solar Photocatalytic Treatment of Dye Pollutants

作者: Ghania Foura , Nawel Chouchou , Ahcène Soualah , Kahina Kouachi , Matteo Guidotti

DOI: 10.3390/CATAL7110344

关键词: AdsorptionCatalysisZeoliteMethylene blueMaterials scienceMicroporous materialDispersion (chemistry)Titanium dioxideNuclear chemistryInorganic chemistryPhotocatalysis

摘要: Zeolite-supported TiO2 and Fe-doped TiO2/zeolite photocatalysts were synthesized, aiming at improving the adsorption properties of microporous support towards polluting dyes photocatalytic performance in treatment adsorbed organics. The TiO2/HY zeolite catalyst exhibited best degradation methylene blue, MB, over 10 wt% under UV light 254 nm. addition Fe species synthesis mixture led to Fe-TiO2/HY catalyst. combination adequate zeolite, good titanium dioxide dispersion, doping a remarkable model dye. Over total removal MB (>98%) was achieved after 60 min very mild conditions simple visible irradiation.

参考文章(70)
José A. Navı́o, Juan J. Testa, Pablo Djedjeian, Javier R. Padrón, Diana Rodrı́guez, Marta I. Litter, Iron-doped titania powders prepared by a sol-gel method. Part II: Photocatalytic properties Applied Catalysis A-general. ,vol. 178, pp. 191- 203 ,(1999) , 10.1016/S0926-860X(98)00286-5
M. B. Suwarnkar, A. N. Kadam, G. V. Khade, N. L. Gavade, K. M. Garadkar, Modification of TiO2 nanoparticles by HZSM-5 for the enhancement in photodegradation of Acid Green 25 Journal of Materials Science: Materials in Electronics. ,vol. 27, pp. 843- 851 ,(2016) , 10.1007/S10854-015-3825-2
Dorian A. H. Hanaor, Charles C. Sorrell, Sand supported mixed-phase TiO2 photocatalysts for water decontamination applications. Advanced Engineering Materials. ,vol. 16, pp. 248- 254 ,(2014) , 10.1002/ADEM.201300259
Yiming Xu, Wei Zheng, Weiping Liu, Enhanced photocatalytic activity of supported TiO2: dispersing effect of SiO2 Journal of Photochemistry and Photobiology A-chemistry. ,vol. 122, pp. 57- 60 ,(1999) , 10.1016/S1010-6030(98)00470-5
Mathias Strauss, Murilo Pastorello, Fernando A Sigoli, Juliana M de Souza e Silva, Italo O Mazali, None, Singular effect of crystallite size on the charge carrier generation and photocatalytic activity of nano-TiO2 Applied Surface Science. ,vol. 319, pp. 151- 157 ,(2014) , 10.1016/J.APSUSC.2014.06.071
Qinghong Zhang, Wugang Fan, Lian Gao, Anatase TiO2 nanoparticles immobilized on ZnO tetrapods as a highly efficient and easily recyclable photocatalyst Applied Catalysis B-environmental. ,vol. 76, pp. 168- 173 ,(2007) , 10.1016/J.APCATB.2007.05.024
Masakazu Anpo, Hiromi Yamashita, Yuichi Ichihashi, Yo Fujii, Miwa Honda, Photocatalytic Reduction of CO2with H2O on Titanium Oxides Anchored within Micropores of Zeolites:  Effects of the Structure of the Active Sites and the Addition of Pt The Journal of Physical Chemistry B. ,vol. 101, pp. 2632- 2636 ,(1997) , 10.1021/JP962696H
Luminita Andronic, Anca Duta, TiO2 thin films for dyes photodegradation Thin Solid Films. ,vol. 515, pp. 6294- 6297 ,(2007) , 10.1016/J.TSF.2006.11.150
Shaobin Wang, Huiting Li, Sujuan Xie, Shenglin Liu, Longya Xu, Physical and chemical regeneration of zeolitic adsorbents for dye removal in wastewater treatment Chemosphere. ,vol. 65, pp. 82- 87 ,(2006) , 10.1016/J.CHEMOSPHERE.2006.02.043