Ultrafast response of third-order optical nonlinearity in glasses containing Bi_2O_3
作者： Naoki Sugimoto , Kazuyuki Hirao , Hirohisa Kanbara , Seiji Fujiwara , Koichiro Tanaka
DOI: 10.1364/OL.21.001637
关键词: Nonlinear optics 、 High harmonic generation 、 Refractive index 、 Optics 、 Laser 、 Four-wave mixing 、 Femtosecond 、 Polarization (waves) 、 Materials science 、 Ultrashort pulse 、 Atomic and Molecular Physics, and Optics
摘要: We prepared nonresonant-type homogeneous glasses containing Bi2O3 by the melting method. The third-order optical nonlinear susceptibility χ(3) was found harmonic generation measurement to be 9.3 × 10−12 esu. attribute nonlinearity of these large molar refraction Bi2O3. These also exhibited an ultrafast response time below 200 fs a degenerate four-wave mixing method using femtosecond laser, indicating that originated mainly from pure electronic polarization.
osapublishing.org
harvard.edu参考文章(12)
Hideki Kobayashi, Hirohisa Kanbara, Masanori Koga, Ken’ichi Kubodera, Third‐order nonlinear optical properties of As2S3 chalcogenide glass Journal of Applied Physics. ,vol. 74, pp. 3683- 3687 ,(1993) , 10.1063/1.354511
Hiroyuki Nasu, Yoshikazu Ibara, Ken'ichi Kubodera, Optical third-harmonic generation from some high-index glasses Journal of Non-crystalline Solids. ,vol. 110, pp. 229- 234 ,(1989) , 10.1016/0022-3093(89)90263-9
E. P. Ippen, C. V. Shank, Picosecond response of a high−repetition−rate CS2 optical Kerr gate Applied Physics Letters. ,vol. 26, pp. 92- 93 ,(1975) , 10.1063/1.88092
Hiroyuki Nasu, Jun Matsuoka, Kanichi Kamiya, Second- and third-order optical non-linearity of homogeneous glasses Journal of Non-crystalline Solids. ,vol. 178, pp. 23- 30 ,(1994) , 10.1016/0022-3093(94)90260-7
D. W. Hall, M. A. Newhouse, N. F. Borrelli, W. H. Dumbaugh, D. L. Weidman, Nonlinear optical susceptibilities of high‐index glasses Applied Physics Letters. ,vol. 54, pp. 1293- 1295 ,(1989) , 10.1063/1.100697
Fumiaki Miyaji, Toshinobu Yoko, Jisun Jin, Sumio Sakka, Toshiharu Fukunaga, Masakatsu Misawa, Neutron and X-ray diffraction studies of PbOGa2O3 and Bi2O3Ga2O3 glasses Journal of Non-crystalline Solids. ,vol. 175, pp. 211- 223 ,(1994) , 10.1016/0022-3093(94)90013-2
E.M. Vogel, S.G. Kosinski, D.M. Krol, J.L. Jackel, S.R. Friberg, M.K. Oliver, J.D. Powers, Structural and optical study of silicate glasses for nonlinear optical devices Journal of Non-crystalline Solids. ,vol. 107, pp. 244- 250 ,(1989) , 10.1016/0022-3093(89)90469-9
Hiroyuki Nasu, Tomoyoshi Uchigaki, Kanichi Kamiya, Hirohisa Kanbara, Ken'ichi Kubodera, Nonresonant-Type Third-order Nonlinearity of (PbO, Nb2O5)-TiO2-TeO2Glass Measured by Third-Harmonic Generation Japanese Journal of Applied Physics. ,vol. 31, pp. 3899- 3900 ,(1992) , 10.1143/JJAP.31.3899
Hiroyuki Nasu, Kenichi Kubodera, Masaki Kobayashi, Maki Nakamura, Kanichi Kamiya, Third‐Harmonic Generation from Some Chalcogenide Glasses Journal of the American Ceramic Society. ,vol. 73, pp. 1794- 1796 ,(1990) , 10.1111/J.1151-2916.1990.TB09838.X
Fumiaki Miyaji, Kiyoharu Tadanaga, Sumio Sakka, Third harmonic generation from MOx-PbO-GaO1.5 ternary glasses Applied Physics Letters. ,vol. 60, pp. 2060- 2061 ,(1992) , 10.1063/1.107089