Investigation on reusing water treatment residuals to remedy soil contaminated with multiple metals in Baiyin, China

作者: Changhui Wang , Yuanyuan Zhao , Yuansheng Pei

DOI: 10.1016/J.JHAZMAT.2012.08.034

关键词: MetallurgyCadmiumZincEnvironmental chemistryChromiumSoil waterEnvironmental remediationExtraction (chemistry)AlumChemistryArsenic

摘要: In this work, the remediation of soils contaminated with multiple metals using ferric and alum water treatment residuals (FARs) in Baiyin, China, was investigated. The results fractionation indicated that after soil treated FARs, arsenic (As), lead (Pb), nickel (Ni), zinc (Zn) copper (Cu) could be transformed into more stable forms, i.e., As bound crystalline Fe/Al oxides other oxidable residual forms. However, forms chromium (Cr) cadmium (Cd) were unaffected. Interestingly, due to effect barium (Ba) predominantly mobile bioaccessibility extraction test demonstrated FARs reduced by 25%, followed Cu, Cr, Zn, Ni Pb. Cd Ba increased; particular, there an increase 41% for at end test. conclusion, can used remedy metals, but comprehensive studies are needed before practical applications work.

参考文章(53)
Zhongren Nan, Chuanyan Zhao, Heavy metal concentrations in gray calcareous soils of Baiyin region, Gansu Province, P.R. China Water Air and Soil Pollution. ,vol. 118, pp. 131- 141 ,(2000) , 10.1023/A:1005135618750
J. J. D'Amore, S. R. Al-Abed, K. G. Scheckel, J. A. Ryan, Methods for Speciation of Metals in Soils Journal of Environmental Quality. ,vol. 34, pp. 1707- 1745 ,(2005) , 10.2134/JEQ2004.0014
Rachana Nagar, Dibyendu Sarkar, Konstantinos C. Makris, Rupali Datta, Victor L. Sylvia, Bioavailability and Bioaccessibility of Arsenic in a Soil Amended with Drinking-Water Treatment Residuals Archives of Environmental Contamination and Toxicology. ,vol. 57, pp. 755- 766 ,(2009) , 10.1007/S00244-009-9318-7
M. C. Chuan, G. Y. Shu, J. C. Liu, Solubility of heavy metals in a contaminated soil: Effects of redox potential and pH Water Air and Soil Pollution. ,vol. 90, pp. 543- 556 ,(1996) , 10.1007/BF00282668
Guangren Qian, Wei Chen, Teik Thye Lim, Pengcheong Chui, In-situ stabilization of Pb, Zn, Cu, Cd and Ni in the multi-contaminated sediments with ferrihydrite and apatite composite additives. Journal of Hazardous Materials. ,vol. 170, pp. 1093- 1100 ,(2009) , 10.1016/J.JHAZMAT.2009.05.093
Rudy Syah Putra, Shunitz Tanaka, Aluminum drinking water treatment residuals (Al-WTRs) as an entrapping zone for lead in soil by electrokinetic remediation Separation and Purification Technology. ,vol. 79, pp. 208- 215 ,(2011) , 10.1016/J.SEPPUR.2011.02.015
Z. Nan, G. Cheng, Copper and zinc uptake by spring wheat (Triticum aestivum L.) and corn (Zea mays L.) grown in Baiyin region. Bulletin of Environmental Contamination and Toxicology. ,vol. 67, pp. 83- 90 ,(2001) , 10.1007/S001280094
Yantao Song, Peter J. Swedlund, Naresh Singhal, Simon Swift, Cadmium(II) speciation in complex aquatic systems: a study with ferrihydrite, bacteria, and an organic ligand. Environmental Science & Technology. ,vol. 43, pp. 7430- 7436 ,(2009) , 10.1021/ES901434V
Jeffrey R. Bacon, Christine M. Davidson, Is there a future for sequential chemical extraction Analyst. ,vol. 133, pp. 25- 46 ,(2008) , 10.1039/B711896A