Fate of a broad spectrum of perfluorinated compounds in soils and biota from Tierra del Fuego and Antarctica

作者: Marta Llorca , Marinella Farré , Máximo Sebastián Tavano , Bruno Alonso , Gabriel Koremblit

DOI: 10.1016/J.ENVPOL.2011.10.027

关键词: Environmental sciencePerfluorooctaneSoil waterBioaccumulationTierraEnvironmental chemistryDeposition (aerosol physics)AlgaeGuanoBiota

摘要: Abstract In this study, the presence of 18 perfluorinated compounds was investigated in biota and environmental samples from Antarctica Tierra de Fuego, which were collected during a sampling campaign carried out along February March 2010. 61 analysed including fish, superficial soils, guano, algae, dung tissues Papua penguin by liquid chromatography coupled to tandem mass spectrometry. The concentrations PFCs ranging 0.10 240 ng/g for most except dung, presented levels between 95 603 ng/g perfluorooctane sulfonate, guano Ushuaia, with concentration 1190–2480 ng/g perfluorohexanoic acid. acids presented, general, highest perfluorooctanesulfonate frequently found compound. present study provides significant amount results, globally supports previous studies, related transport, deposition, biodegradation bioaccumulation patterns PFCs.

参考文章(53)
Bryan Boulanger, John Vargo, Jerald L. Schnoor, Keri C. Hornbuckle, Detection of perfluorooctane surfactants in Great Lakes water. Environmental Science & Technology. ,vol. 38, pp. 4064- 4070 ,(2004) , 10.1021/ES0496975
Craig M. Butt, Derek C. G. Muir, Ian Stirling, Michael Kwan, Scott A. Mabury, Rapid Response of Arctic Ringed Seals to Changes in Perfluoroalkyl Production Environmental Science & Technology. ,vol. 41, pp. 42- 49 ,(2007) , 10.1021/ES061267M
Annekatrin Dreyer, Ingo Weinberg, Christian Temme, Ralf Ebinghaus, Polyfluorinated compounds in the atmosphere of the Atlantic and Southern Oceans: evidence for a global distribution. Environmental Science & Technology. ,vol. 43, pp. 6507- 6514 ,(2009) , 10.1021/ES9010465
Konstantinos Prevedouros, Ian T. Cousins, Robert C. Buck, Stephen H. Korzeniowski, Sources, fate and transport of perfluorocarboxylates. Environmental Science & Technology. ,vol. 40, pp. 32- 44 ,(2006) , 10.1021/ES0512475
M. Shoeib, T. Harner, P. Vlahos, Perfluorinated chemicals in the arctic atmosphere. Environmental Science & Technology. ,vol. 40, pp. 7577- 7583 ,(2006) , 10.1021/ES0618999
Brian F. Scott, Christine Spencer, Scott A. Mabury, Derek C. G. Muir, Poly and Perfluorinated Carboxylates in North American Precipitation Environmental Science & Technology. ,vol. 40, pp. 7167- 7174 ,(2006) , 10.1021/ES061403N
John P. Giesy, Kurunthachalam Kannan, Global distribution of perfluorooctane sulfonate in wildlife. Environmental Science & Technology. ,vol. 35, pp. 1339- 1342 ,(2001) , 10.1021/ES001834K
Kurt R. Rhoads, Elisabeth M.-L. Janssen, Richard G. Luthy, Craig S. Criddle, Aerobic Biotransformation and Fate of N-Ethyl Perfluorooctane Sulfonamidoethanol (N-EtFOSE) in Activated Sludge Environmental Science & Technology. ,vol. 42, pp. 2873- 2878 ,(2008) , 10.1021/ES702866C
Annika Jahnke, Urs Berger, Ralf Ebinghaus, Christian Temme, Latitudinal Gradient of Airborne Polyfluorinated Alkyl Substances in the Marine Atmosphere between Germany and South Africa (53° N−33° S) Environmental Science & Technology. ,vol. 41, pp. 3055- 3061 ,(2007) , 10.1021/ES062389H