Ultrasonic-assisted synthesis of mesoporous g-C3N4/Na-bentonite composites and its application for efficient photocatalytic simultaneous removal of Cr(VI) and RhB

作者: Yadan Guo , Chenxi Li , Yiqin Guo , Xuegang Wang , Xiaomeng Li

DOI: 10.1016/J.COLSURFA.2019.123624

关键词: PhotocatalysisGraphitic carbon nitrideX-ray photoelectron spectroscopyComposite materialComposite numberAdsorptionNanocompositeNitrideMaterials scienceMesoporous material

摘要: Abstract Graphitic carbon nitride (g-C3N4) is a new type of nonmetal polymeric semiconductor photocatalyst for removal pollutants. To overcome the low BET surface and electron–hole recombination rate g-C3N4 photocatalysts, we successfully synthesized g-C3N4/Na-bentonite composites using an ultrasonic-assisted method. The XRD showed that composite was composed Na-bentonite. analyses TEM XPS indicated graphite intercalated on Na-bentonite via strategy, nanocomposites presented remarkable light absorption capacities mesoporous structure observed by UV–vis DRS In addition, as-prepared can be used photocatalytic single RhB or Cr(VI), efficiencies Cr(VI) reduction are increased from 53.2% to 88.6% in RhB/Cr(VI) mix-system. Superior stability high were also exhibited up 4 cycles. enhancement due strong adsorption higher charge separation efficiency composites.

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