Enhanced catalytic activity of Fe bimetallic modified PAN fiber complexes prepared with different assisted metal ions for degradation of organic dye
作者： Yongchun Dong , Zhenbang Han , Siming Dong , Jinna Wu , Zhizhong Ding
DOI: 10.1016/J.CATTOD.2011.04.026
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摘要: Abstract Two transition metal ions (Cu2+ and Co2+) two rare earth (Ce3+ La3+) were used as the assisted ions, respectively to prepare Fe bimetallic amidoximated polyacrylonitrile (AO-PAN) fiber complexes. And their coordination configuration visible light adsorption properties examined by number determination UV–vis–DRS. Then catalytic performance of these complexes was evaluated heterogeneous Fenton catalysts in Rhodamine B degradation changing nature dosage added. The results indicated that incorporation led AO-PAN with more unsaturated configurations than monometallic complex due changes numbers. Cu–Fe or Ce–Fe varied significantly Cu/Fe Ce/Fe molar ratio. showed a higher toward dye complex. can affect activities. found have better stability wider pH range
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S.H. Bossmann, E. Oliveros, S. Göb, M. Kantor, A. Göppert, L. Lei, P.L. Yue, A.M. Braun, Degradation of polyvinyl alcohol (PVA) by homogeneous and heterogeneous photocatalysis applied to the photochemically enhanced Fenton reaction. Water Science and Technology. ,vol. 44, pp. 257- 262 ,(2001) , 10.2166/WST.2001.0300
Horst Kunkely, Arnd Vogler, Photoredox reaction of with PctsH2=phthalocyaninetetrasulfonate induced by peroxide to Fe(III) charge transfer excitation Inorganica Chimica Acta. ,vol. 358, pp. 4086- 4088 ,(2005) , 10.1016/J.ICA.2005.04.045
Geoffrey Wilkinson, Paul L. Gaus, F. Albert Cotton, Basic Inorganic Chemistry ,(1976)
Mugunthu R. Dhananjeyan, John Kiwi, Peter Albers, Octav Enea, Photo-Assisted ImmobilizedFenton Degradation up to pH 8 of Azo Dye Orange II Mediated by Fe3+/Nafion/Glass Fibers Helvetica Chimica Acta. ,vol. 84, pp. 3433- 3445 ,(2001) , 10.1002/1522-2675(20011114)84:11<3433::AID-HLCA3433>3.0.CO;2-A
J. Fernandez, J. Bandara, A. Lopez, Ph. Buffat, J. Kiwi, Photoassisted Fenton Degradation of Nonbiodegradable Azo Dye (Orange II) in Fe-Free Solutions Mediated by Cation Transfer Membranes Langmuir. ,vol. 15, pp. 185- 192 ,(1999) , 10.1021/LA980382A
Iara R. Guimaraes, Amanda Giroto, Luiz C.A. Oliveira, Mario C. Guerreiro, Diana Q. Lima, José D. Fabris, Synthesis and thermal treatment of cu-doped goethite: Oxidation of quinoline through heterogeneous fenton process Applied Catalysis B-environmental. ,vol. 91, pp. 581- 586 ,(2009) , 10.1016/J.APCATB.2009.06.030
Yongchun Dong, Zhenbang Han, Chunyan Liu, Fang Du, Preparation and photocatalytic performance of Fe (III)-amidoximated PAN fiber complex for oxidative degradation of azo dye under visible light irradiation. Science of The Total Environment. ,vol. 408, pp. 2245- 2253 ,(2010) , 10.1016/J.SCITOTENV.2010.01.020
Jiyun Feng, Xijun Hu, Po Lock Yue, Huai Yong Zhu, Gao Qing Lu, None, Degradation of Azo-dye Orange II by a Photoassisted Fenton Reaction Using a Novel Composite of Iron Oxide and Silicate Nanoparticles as a Catalyst Industrial & Engineering Chemistry Research. ,vol. 42, pp. 2058- 2066 ,(2003) , 10.1021/IE0207010
Yannick Jeanvoine, Riccardo Spezia, Mn2+-, Fe2+-, Co2+-, Ni2+-, Cu2+-, and Zn2+-binding chalcogen-chalcogen bridges: a compared MP2 and B3LYP study. Journal of Physical Chemistry A. ,vol. 113, pp. 7878- 7887 ,(2009) , 10.1021/JP811460F
Lei Li, Jing Jin, Zhongfeng Shi, Limin Zhao, Jiacao Liu, Yongheng Xing, Shuyun Niu, Cd (II)–M (II) hetero-nuclear coordination polymers: Synthesis, structure and photo-electric properties (M=Fe, Co, Cd) Inorganica Chimica Acta. ,vol. 363, pp. 748- 754 ,(2010) , 10.1016/J.ICA.2009.11.036