Highly stable CsPbBr3 perovskite quantum dots incorporated in aluminum stearate

作者: Leilei Chen , Xiaopeng Cheng , Dabin Yu , Jinhua Zhang , Yajing Chang

DOI: 10.1016/J.JLUMIN.2021.117962

关键词:

摘要: Abstract CsPbBr3 perovskite quantum dots (PQDs) have drawn much attention for their high photoluminescence yield and great potential in optoelectronic applications. However, they suffer from poor stability under humid condition. This paper reports PQDs incorporated aluminum stearate (AlSt3) matrix via an improved co-precipitation approach, which AlSt3 not only acted as hydrophobic to protect surrounding environment, but also passivated the surface of coordination bond St-Cs St-Pb, well between Al3+ Br−. By this method, as-synthesized CsPbBr3-AlSt3 composites exhibited excellent ambient condition even directly water more than 60 days. With (green emission) used color-conversion layer, a white light-emitting diode (WLED) was fabricated with color rendering index (Ra) 90 low temperature (Tc) 4929 K. These results suggest that method pave effective way stabilize PQDs, is importance further application.

参考文章(35)
S. Ye, F. Xiao, Y.X. Pan, Y.Y. Ma, Q.Y. Zhang, Phosphors in phosphor-converted white light-emitting diodes: Recent advances in materials, techniques and properties Materials Science & Engineering R-reports. ,vol. 71, pp. 1- 34 ,(2010) , 10.1016/J.MSER.2010.07.001
Hongyan Duan, Yang Jiang, Yugang Zhang, Dapeng Sun, Chao Liu, Jian Huang, Xinzheng Lan, Hongyang Zhou, Lei Chen, Honghai Zhong, High quantum-yield CdSexS1-x/ZnS core/shell quantum dots for warm white light-emitting diodes with good color rendering. Nanotechnology. ,vol. 24, pp. 285201- ,(2013) , 10.1088/0957-4484/24/28/285201
Jizhong Song, Jianhai Li, Xiaoming Li, Leimeng Xu, Yuhui Dong, Haibo Zeng, Nanocrystals: Quantum Dot Light-Emitting Diodes Based on Inorganic Perovskite Cesium Lead Halides (CsPbX3) (Adv. Mater. 44/2015) Advanced Materials. ,vol. 27, pp. 7161- 7161 ,(2015) , 10.1002/ADMA.201570302
Parthiban Ramasamy, Da-Hye Lim, Bumjin Kim, Seung-Ho Lee, Min-Sang Lee, Jong-Soo Lee, All-inorganic cesium lead halide perovskite nanocrystals for photodetector applications Chemical Communications. ,vol. 52, pp. 2067- 2070 ,(2016) , 10.1039/C5CC08643D
Hung-Chia Wang, Shin-Ying Lin, An-Cih Tang, Bheeshma Pratap Singh, Hung-Chun Tong, Ching-Yi Chen, Yu-Chun Lee, Tzong-Liang Tsai, Ru-Shi Liu, Mesoporous Silica Particles Integrated with All-Inorganic CsPbBr3 Perovskite Quantum-Dot Nanocomposites (MP-PQDs) with High Stability and Wide Color Gamut Used for Backlight Display. Angewandte Chemie. ,vol. 55, pp. 7924- 7929 ,(2016) , 10.1002/ANIE.201603698
Georgian Nedelcu, Loredana Protesescu, Sergii Yakunin, Maryna I. Bodnarchuk, Matthias J. Grotevent, Maksym V. Kovalenko, Fast Anion-Exchange in Highly Luminescent Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, I) Nano Letters. ,vol. 15, pp. 5635- 5640 ,(2015) , 10.1021/ACS.NANOLETT.5B02404
Longfei Lv, Yibing Xu, Hehai Fang, Wenjin Luo, Fangjie Xu, Limin Liu, Biwei Wang, Xianfeng Zhang, Dong Yang, Weida Hu, Angang Dong, Generalized colloidal synthesis of high-quality, two-dimensional cesium lead halide perovskite nanosheets and their applications in photodetectors Nanoscale. ,vol. 8, pp. 13589- 13596 ,(2016) , 10.1039/C6NR03428D
Yongping Fu, Haiming Zhu, Constantinos C. Stoumpos, Qi Ding, Jue Wang, Mercouri G. Kanatzidis, Xiaoyang Zhu, Song Jin, Broad Wavelength Tunable Robust Lasing from Single-Crystal Nanowires of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, I) ACS Nano. ,vol. 10, pp. 7963- 7972 ,(2016) , 10.1021/ACSNANO.6B03916
Vikash Kumar Ravi, Ganesh B. Markad, Angshuman Nag, Band Edge Energies and Excitonic Transition Probabilities of Colloidal CsPbX3 (X = Cl, Br, I) Perovskite Nanocrystals ACS energy letters. ,vol. 1, pp. 665- 671 ,(2016) , 10.1021/ACSENERGYLETT.6B00337
Chun Sun, Yu Zhang, Cheng Ruan, Chunyang Yin, Xiaoyong Wang, Yiding Wang, William W. Yu, Efficient and Stable White LEDs with Silica‐Coated Inorganic Perovskite Quantum Dots Advanced Materials. ,vol. 28, pp. 10088- 10094 ,(2016) , 10.1002/ADMA.201603081