Lévy statistics of vibrational mode fluctuations of single molecules from surface-enhanced Raman scattering.
作者： Anna Rita Bizzarri , Salvatore Cannistraro
DOI: 10.1103/PHYSREVLETT.94.068303
关键词:
摘要: Surface-enhanced Raman spectra of a single Fe-protoporphyrin IX molecule display drastic fluctuations in frequency and intensity. When analyzed their temporal evolution, the vibrational modes undergo an on-off switching behavior that is shown to follow Levy statistics. Such time dependent process may encode both dynamics molecule-environment interactions intrinsic gating or activation mode emission mechanism.
unirioja.es
harvard.edu
sci-hub.se 参考文章(29)
Uriel Frisch, Micheal F. Shlesinger, George M. Zaslavsky, Lévy Flights and Related Topics in Physics ,(2013)
William Feller, An introduction to probability theory and its applications ,(1950)
J. A. Veerman, M. F. Garcia-Parajo, L. Kuipers, N. F. van Hulst, Time-varying triplet state lifetimes of single molecules Physical Review Letters. ,vol. 83, pp. 2155- 2158 ,(1999) , 10.1103/PHYSREVLETT.83.2155
Xavier Brokmann, J-P Hermier, Gaëtan Messin, Pierre Desbiolles, J-P Bouchaud, Maxime Dahan, None, Statistical aging and nonergodicity in the fluorescence of single nanocrystals. Physical Review Letters. ,vol. 90, pp. 120601- ,(2003) , 10.1103/PHYSREVLETT.90.120601
E. Barkai, R. Silbey, G. Zumofen, Levy distribution of single molecule line shape cumulants in glasses Physical Review Letters. ,vol. 84, pp. 5339- 5342 ,(2000) , 10.1103/PHYSREVLETT.84.5339
E. Barkai, A. V. Naumov, Yu. G. Vainer, M. Bauer, L. Kador, Lévy statistics for random single-molecule line shapes in a glass. Physical Review Letters. ,vol. 91, pp. 075502- ,(2003) , 10.1103/PHYSREVLETT.91.075502
Eli Barkai, YounJoon Jung, Robert Silbey, Theory of single-molecule spectroscopy: beyond the ensemble average. Annual Review of Physical Chemistry. ,vol. 55, pp. 457- 507 ,(2004) , 10.1146/ANNUREV.PHYSCHEM.55.111803.143246
Shuming Nie, Steven R Emory, Probing Single Molecules and Single Nanoparticles by Surface-Enhanced Raman Scattering Science. ,vol. 275, pp. 1102- 1106 ,(1997) , 10.1126/SCIENCE.275.5303.1102
Katrin Kneipp, Yang Wang, Harald Kneipp, Lev T. Perelman, Irving Itzkan, Ramachandra R. Dasari, Michael S. Feld, Single Molecule Detection Using Surface-Enhanced Raman Scattering (SERS) Physical Review Letters. ,vol. 78, pp. 1667- 1670 ,(1997) , 10.1103/PHYSREVLETT.78.1667
Mikael Käll, Lars Börjesson, Hongxing Xu, Erik J. Bjerneld, Spectroscopy of Single Hemoglobin Molecules by Surface Enhanced Raman Scattering Physical Review Letters. ,vol. 83, pp. 4357- 4360 ,(1999) , 10.1103/PHYSREVLETT.83.4357