Track size and track structure in polymer irradiated by heavy ions

作者: P Apel , A Schulz , R Spohr , C Trautmann , V Vutsadakis

DOI: 10.1016/S0168-583X(98)00445-5

关键词:

摘要: The structure of latent tracks in polyethylene terephthalate (PET) was studied using chemical etching combined with a conductometric technique. Polymer samples were irradiated Ar, Kr, Xe, Au, and U ions energies the range 1 to 11.6 MeV/u. kinetics investigated radii 0–100 nm. highly damaged track core manifests itself on curves as zone where etch rate changes dramatically reaches its minimum at radius few It found that is approximately proportional (dE/dx)0.55. surrounded by halo. In halo proceeds slowly increases approaching constant value. Cross linking macromolecules causes reduction which extends up distances exceeding 100 nm case heaviest ions. Measurable change such large could not be predicted from shape calculated spatial distributions energy dissipated tracks. Obviously, formation extended influenced diffusion active intermediates polymer bulk.

参考文章(15)
P. Apel, N. Angert, W. Brüchle, H. Hermann, U. Kampschulte, P. Klein, L.I. Kravets, Yu.Ts. Oganessian, G. Remmert, R. Spohr, T. Steckenreiter, C. Trautmann, J. Vetter, Solvent induced track sensitization. Extraction of oligomers Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms. ,vol. 86, pp. 325- 332 ,(1994) , 10.1016/0168-583X(94)95297-3
V. Chailley, E. Dooryhée, S. Bouffard, E. Balanzat, M. Levalois, Observations by X-ray diffraction of structural changes in mica irradiated by swift heavy ions Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms. ,vol. 91, pp. 162- 167 ,(1994) , 10.1016/0168-583X(94)96208-1
J. Ackermann, N. Angert, R. Neumann, C. Trautmann, M. Dischner, T. Hagen, M. Sedlacek, Ion track diameters in mica studied with scanning force microscopy Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms. ,vol. 107, pp. 181- 184 ,(1996) , 10.1016/0168-583X(95)01037-8
M. Toulemonde, S. Bouffard, F. Studer, Swift heavy ions in insulating and conducting oxides: tracks and physical properties Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms. ,vol. 91, pp. 108- 123 ,(1994) , 10.1016/0168-583X(94)96200-6
F. Thibaudau, J. Cousty, E. Balanzat, S. Bouffard, Atomic-force-microscopy observations of tracks induced by swift Kr ions in mica. Physical Review Letters. ,vol. 67, pp. 1582- 1585 ,(1991) , 10.1103/PHYSREVLETT.67.1582
C. P. Bean, M. V. Doyle, G. Entine, Etching of Submicron Pores in Irradiated Mica Journal of Applied Physics. ,vol. 41, pp. 1454- 1459 ,(1970) , 10.1063/1.1659056
P. Apel, A. Schulz, R. Spohr, C. Trautmann, V. Vutsadakis, Tracks of very heavy ions in polymers Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms. ,vol. 131, pp. 55- 63 ,(1997) , 10.1016/S0168-583X(97)00389-3
F Petersen, W Enge, Energy loss dependent transversal etching rates of heavy ion tracks in plastic Radiation Measurements. ,vol. 25, pp. 43- 46 ,(1995) , 10.1016/1350-4487(95)00028-D
S. Bouffard, J. Cousty, Y. Pennec, F. Thibaudau, STM and AFM observations of latent tracks Radiation Effects and Defects in Solids. ,vol. 126, pp. 225- 228 ,(1993) , 10.1080/10420159308219714