Increasing gas-solids mass transfer in fluidized beds by application of confined fluidization-A feasibility study

作者: Jesper Aronsson , David Pallarès , Magnus Rydén , Anders Lyngfelt

DOI: 10.3390/APP9040634

关键词:

摘要: Fluidized bed applications where the material plays an active role in chemical reactions, e.g. looping combustion, have seen increase interest over past decade. When these processes are to be scaled up industrial or utility scale mass transfer between gas and solids phases can become a limitation for conversion. Confined fluidized beds were conceptualized other purposes 1960's but yet applied recent technologies. Here it is investigated if they prove useful also feasible from perspectives such as pressure drop throughflow. Four spherical packing solids, 6.35-25.4 mm diameter at two different densities, tested. For experiments fluidizing air was humidified water adsorption rate onto silica gel particles acting measured. Olivine sand used further measuring segregation of packing, maximum vertical crossflow solids. It found that increased by factor 1.9-3.8 with compared non-packed reference. With high-density voidage inside 58% higher than conventional bed. Low density favoured its flotsam fluidization velocities yield better mixing Maximum cross-flow significantly low fluidized, stationary packing. Conclusively, prospect using confined improving looks promising both performance practical standpoints.

参考文章(18)
S. Sircar, M.B. Rao, T.C. Golden, Chapter 2.12 Drying of gases and liquids by activated alumina Studies in Surface Science and Catalysis. ,vol. 99, pp. 629- 646 ,(1996) , 10.1016/S0167-2991(06)81038-4
Diana Carolina Guío-Pérez, Hermann Hofbauer, Tobias Pröll, Effect of ring‐type internals on solids distribution in a dual circulating fluidized bed system—cold flow model study Aiche Journal. ,vol. 59, pp. 3612- 3623 ,(2013) , 10.1002/AIC.14120
D. Ziółkowski, J. Michalski, Onset of fluidization of fines in an organized system within voids of packings formed of spherical elements Chemical Engineering Science. ,vol. 47, pp. 4007- 4016 ,(1992) , 10.1016/0009-2509(92)85150-A
G. Donsì, G. Ferrari, B. Formisani, G. Longo, Confined fluidization of fine particles in a packed bed of coarse particles: Model and experimental description Powder Technology. ,vol. 61, pp. 75- 85 ,(1990) , 10.1016/0032-5910(90)80068-A
T. Hoffmann, A. Hailu Bedane, M. Peglow, E. Tsotsas, M. Jacob, Particle–Gas Mass Transfer in a Spouted Bed with Adjustable Air Inlet Drying Technology. ,vol. 29, pp. 257- 265 ,(2011) , 10.1080/07373937.2010.483046
J. P. Sutherland, George Vassilatos, Hiroshi Kubota, G. L. Osberg, The effect of packing on a fluidized bed Aiche Journal. ,vol. 9, pp. 437- 441 ,(1963) , 10.1002/AIC.690090406
JR Grace, R Clift, None, On the two-phase theory of fluidization Chemical Engineering Science. ,vol. 29, pp. 327- 334 ,(1974) , 10.1016/0009-2509(74)80039-4
G. Donsì, G. Ferrari, B. Formisani, Expansion behaviour of confined fluidized beds of fine particles Canadian Journal of Chemical Engineering. ,vol. 67, pp. 185- 190 ,(1989) , 10.1002/CJCE.5450670204
D. Mandal, M. Vinjamur, D. Sathiyamoorthy, Hydrodynamics of beds of small particles in the voids of coarse particles Powder Technology. ,vol. 235, pp. 256- 262 ,(2013) , 10.1016/J.POWTEC.2012.10.029