Effect of resonance dipole-dipole interaction on spectra of adsorbed SF6 molecules.
作者： Anna N Dobrotvorskaia , Tatiana D Kolomiitsova , Sergey N Petrov , Dmitriy N Shchepkin , Konstantin S Smirnov
DOI: 10.1016/J.SAA.2015.04.002
关键词:
摘要: Abstract Adsorption of SF6 on zinc oxide and silicalite-1 was investigated by a combination IR spectroscopy with the calculations spectra means modernized model, developed previously for liquids. Comparison experimental results modeling shows that complex band shapes in adsorbed molecules extremely high absorbance are due to strong resonance dipole–dipole interaction (RDDI) rather surface heterogeneity or presence specific sites. Perfect agreement between calculated observed found ZnO, while some dissimilarity intensities attributed complicated geometry molecular arrangement channels.
harvard.edu
elsevier.com
sci-hub.se 参考文章(34)
D. A. King, Coupling Induced Vibrational Frequency Shifts and Island Size Determination: CO on Pt {001} and Pt {111} Springer, Berlin, Heidelberg. pp. 179- 184 ,(1980) , 10.1007/978-3-642-88644-7_11
Kazuo Nakamoto, Infrared spectra of inorganic and coordination compounds Wiley-Interscience. ,(1963)
T.J. Chuang, H. Seki, Ingo Hussla, Infrared photodesorption: Vibrational excitation and energy transfer processes on surfaces Surface Science Letters. ,vol. 158, pp. 525- 552 ,(1985) , 10.1016/0039-6028(85)90329-2
AA Tsyganenko, SM Zverev, None, Mechanism of lateral interactions between molecules adsorbed on oxide surfaces Reaction Kinetics and Catalysis Letters. ,vol. 36, pp. 269- 274 ,(1988) , 10.1007/BF02063817
Thomas K. Sherwood, Robert E. Street, Robert C. Reid, The Properties of Gases and Liquids ,(1977)
D. Scarano, G. Spoto, A. Zecchina, A. Reller, Relations between the morphology of ZnO microcrystals and their adsorptive properties towards CO as studied by IR spectroscopy Surface Science. ,vol. 211, pp. 1012- 1017 ,(1989) , 10.1016/0039-6028(89)90868-6
JC Lavalley, J Saussey, AA Tsyganenko, None, IR study of interactions between different molecules CO-adsorbed on ZnO Surface Science. ,vol. 315, pp. 112- 118 ,(1994) , 10.1016/0039-6028(94)90547-9
Chifuru Noda, Hugh H. Richardson, George E. Ewing, Infrared spectroscopy of CO on NaCl(100). II. Vibrational dephasing and band shapes Journal of Chemical Physics. ,vol. 92, pp. 2099- 2105 ,(1990) , 10.1063/1.458042
J. Heidberg, K.-W. Stahmer, H. Stein, H. Weiss, Linear infrared spectra and laser-induced resonant desorption in the coadsorbate 12C16O/13C16O - NaCl Journal of Electron Spectroscopy and Related Phenomena. ,vol. 45, pp. 87- 98 ,(1987) , 10.1016/0368-2048(87)80057-9
D. Scarano, G. Spoto, S. Bordiga, A. Zecchina, C. Lamberti, Lateral interactions in CO adlayers on prismatic ZnO faces: a FTIR and HRTEM study Surface Science. ,vol. 276, pp. 281- 298 ,(1992) , 10.1016/0039-6028(92)90716-J