Examination of the Optimized Conditions for the Conversion of NOX Pollution in DBD Plasma Reactor

作者: R Yarahmadi , M R Omidkhah , S B Mortazavi , P Moridi , Asilian Hasan

DOI: 10.30492/IJCCE.2010.9910

关键词:

摘要: Since NOx family, one of the most important causes air pollution, is primary source acid rains, ozone layer depletion, and breathing disorders, mitigation these pollutants now a global concern. In off-gases internal combustion engines running with oxygen excess, non-thermal plasmas (NTPs) have an oxidative potential, which results in effective conversion NO to NO2. This paper aims at studying methods mitigating eliminating atmospheric condition by means plasma reactors. It examines some key parameters such as temperature, space velocity, voltage, propane/NOx mole ratio. The showed that, velocity 11500-2300 h -1 domain did not show any significant on conversion. Our findings also revealed that optimal conditions for into N2, O2, NO2 are temperature (180 ◦ C), voltage (10 kV), equal ratio propane NOx. this condition, efficiency 78% standard deviation 12% were obtained. N2 O2. (efficiency=53% ) 180 C, 5 kV, 0.3 respectively. Plasma reactor acts primery treatment direct neutral non-poisonous molecules O2 N2.

参考文章(12)
WR Wijnand Rutgers, van Em Eddie Veldhuizen, Corona discharges: fundamentals and diagnostics Eindhoven University of Technology. pp. 40- 49 ,(2001)
Ken Okazaki, Tomohiro Nozaki, Ultrashort pulsed barrier discharges and applications Pure and Applied Chemistry. ,vol. 74, pp. 447- 452 ,(2002) , 10.1351/PAC200274030447
Jinhai Niu, Xuefeng Yang, Aimin Zhu, Lingling Shi, Qi Sun, Yong Xu, Chuan Shi, Plasma-assisted selective catalytic reduction of NOx by C2H2 over Co-HZSM-5 catalyst Catalysis Communications. ,vol. 7, pp. 297- 301 ,(2006) , 10.1016/J.CATCOM.2005.10.016
Mehul P. Patel, T. Terry Ng, Srikanth Vasudevan, Thomas C. Corke, Martiqua L. Post, Thomas E. McLaughlin, Charles F. Suchomel, Scaling Effects of an Aerodynamic Plasma Actuator Journal of Aircraft. ,vol. 45, pp. 223- 236 ,(2008) , 10.2514/1.31830
R. Dorai, K. Hassouni, M.J. Kushner, Consequences of soot particles on the plasma remediation of NO/sub x/ in the presence of hydrocarbons international conference on plasma science. pp. 224- ,(2000) , 10.1109/PLASMA.2000.855050
A Ohl, W Schleinitz, A Meyer-Sievers, A Becker, D Keller, K Schröder, J Conrads, Design of an UHV reactor system for plasma surface treatment of polymer materials Surface & Coatings Technology. ,vol. 116, pp. 1006- 1010 ,(1999) , 10.1016/S0257-8972(99)00139-5
H Miessner, K.-P Francke, R Rudolph, Th Hammer, NOX removal in excess oxygen by plasma-enhanced selective catalytic reduction Catalysis Today. ,vol. 75, pp. 325- 330 ,(2002) , 10.1016/S0920-5861(02)00085-8
J.-O. Chae, Non-thermal plasma for diesel exhaust treatment Journal of Electrostatics. ,vol. 57, pp. 251- 262 ,(2003) , 10.1016/S0304-3886(02)00165-1
A. A. Fridman, V. D. Rusanov, Theoretical basis of non-equilibrium near atmospheric pressure plasma chemistry Pure and Applied Chemistry. ,vol. 66, pp. 1267- 1278 ,(1994) , 10.1351/PAC199466061267
Gui-Bing Zhao, Xudong Hu, Man-Chung Yeung, Ovid A. Plumb, Maciej Radosz, Nonthermal Plasma Reactions of Dilute Nitrogen Oxide Mixtures: NOx in Nitrogen Industrial & Engineering Chemistry Research. ,vol. 43, pp. 2315- 2323 ,(2004) , 10.1021/IE049934C