One-dimensional Thomas-Fermi model of atoms, molecules, and small clusters exposed to an intense laser field

作者: Mirosław Brewczyk , Kazimierz Rza̧żewski

DOI: 10.1103/PHYSREVA.60.2285

关键词:

摘要: We have developed a one-dimensional time-dependent Thomas-Fermi model of atoms, molecules, and small clusters exposed to an intense subpicosecond laser field. In this model, the dynamics electronic cloud is governed by hydrodynamic equations motion, whereas nuclei move in accordance with Newton equations. The quantum mechanics enters approach only through constitutive relation between pressure density, which derived from application Fermi-Dirac statistics noninteracting $T=0$ temperature electron gas. time-independent version formulated terms integral equation for electric potential, also discussed. present numerical results diatomic molecules irradiated strong pulses. case we observe multielectron ionization accompanied dissociation. kinetic energy defect, understood as reduction resulting ions comparison simple Coulomb explosion picture, explained screening effect escaping fragments ejected electrons. For find that cluster has stepwise character; consecutive layers atoms are stripped off one one. highly energetic (as compared systems) atomic even relatively low intensities few clusters. Also, predicts nonuniform distribution among same charge state supports idea hot electrons generated via mechanism inverse bremsstrahlung.

参考文章(40)
T. D. Donnelly, T. Ditmire, K. Neuman, M. D. Perry, R. W. Falcone, High-order harmonic generation in atom clusters. Physical Review Letters. ,vol. 76, pp. 2472- 2475 ,(1996) , 10.1103/PHYSREVLETT.76.2472
Y. L. Shao, T. Ditmire, J. W. G. Tisch, E. Springate, J. P. Marangos, M. H. R. Hutchinson, Multi-keV Electron Generation in the Interaction of Intense Laser Pulses with Xe Clusters. Physical Review Letters. ,vol. 77, pp. 3343- 3346 ,(1996) , 10.1103/PHYSREVLETT.77.3343
T. Ditmire, J. W. G. Tisch, E. Springate, M. B. Mason, N. Hay, J. P. Marangos, M. H. R. Hutchinson, High Energy Ion Explosion of Atomic Clusters: Transition from Molecular to Plasma Behavior Physical Review Letters. ,vol. 78, pp. 2732- 2735 ,(1997) , 10.1103/PHYSREVLETT.78.2732
Mirosław Brewczyk, Charles W. Clark, Maciej Lewenstein, Kazimierz Rza̧żewski, STEPWISE EXPLOSION OF ATOMIC CLUSTERS INDUCED BY A STRONG LASER FIELD Physical Review Letters. ,vol. 80, pp. 1857- 1860 ,(1998) , 10.1103/PHYSREVLETT.80.1857
Christoph G. Rose-Petruck, Kenneth J. Schafer, Christopher P. P. Barty, Possible ionization ignition in laser-driven clusters SPIE's 1995 International Symposium on Optical Science, Engineering, and Instrumentation. ,vol. 2523, pp. 272- 283 ,(1995) , 10.1117/12.220988
C. Rose-Petruck, K. J. Schafer, K. R. Wilson, C. P. J. Barty, Ultrafast electron dynamics and inner-shell ionization in laser driven clusters Physical Review A. ,vol. 55, pp. 1182- 1190 ,(1997) , 10.1103/PHYSREVA.55.1182
K Boyer, B D Thompson, A McPherson, C K Rhodes, Evidence for coherent electron motions in multiphoton X-ray production from Kr and Xe clusters Journal of Physics B. ,vol. 27, pp. 4373- 4389 ,(1994) , 10.1088/0953-4075/27/18/030
T. Ditmire, T. Donnelly, A. M. Rubenchik, R. W. Falcone, M. D. Perry, Interaction of intense laser pulses with atomic clusters. Physical Review A. ,vol. 53, pp. 3379- 3402 ,(1996) , 10.1103/PHYSREVA.53.3379
G. F. Kventsel, J. Katriel, Thomas-Fermi atom inndimensions Physical Review A. ,vol. 24, pp. 2299- 2301 ,(1981) , 10.1103/PHYSREVA.24.2299
P. Hohenberg, W. Kohn, Inhomogeneous Electron Gas Physical Review. ,vol. 136, pp. 864- 871 ,(1964) , 10.1103/PHYSREV.136.B864