A budget analysis of the formation of haze in Beijing

作者: Xuexi Tie , Qiang Zhang , Hui He , Junji Cao , Suqing Han

DOI: 10.1016/J.ATMOSENV.2014.10.038

关键词:

摘要: Abstract During recent winters, hazes often occurred in Beijing, causing major environmental problems. To understand the causes of this “Beijing Haze”, a haze episode (from Oct. 21 to 31, 2013) Beijing was analyzed. episode, daily mean concentration fine particulate matter (PM2.5) reached peak value 270 μg/m3 on 28, 2013, and rapidly decreased 50 μg/m3 next day (Oct. 29, 2013). This strong variability provided good opportunity study Haze”. Two numerical models were applied for study. The first model is chemical/dynamical regional (WRF-Chem). mainly used effects that weather conditions have PM2.5 concentrations region. results show presence high air pressure northwest (NW-High) generally produced winds with clean upwind air. As result, NW-High played an important role cleaning Beijing's PM. However, NW-High's effect did not occur every situation. When there low southeast (SE-Low) accompanied by NW-High, convergent zone appeared Beijing. pollutants became sandwiched, producing second box model, which estimate some crucial parameters associated budget Under calm winds, calculations continuous local emissions accumulate pollutants. 150 μg/m3 250 μg/m3 within one (1) two (2) days, respectively. Without horizontal dilution, can be considered as upper time limit (the fastest time) occurrences events wind speed (WSb) calculated balance between atmospheric processes. WSb strongly dependent planetary boundary layer (PBL) height direction. SE-Low conditions, 2 m/s higher PBL (700 m). under lower heights, increases, reaching 4.5 m/s 7.0 m/s heights 300 m 200 m, In contrast, reduces 2.5 m/s 4.0 m/s. These suggest when prevailing (with speeds >4 m/s), (PM) begins decrease.

参考文章(33)
R. Zhang, J. Jing, J. Tao, S.-C. Hsu, G. Wang, J. Cao, C. S. L. Lee, L. Zhu, Z. Chen, Y. Zhao, Z. Shen, Chemical characterization and source apportionment of PM 2.5 in Beijing: seasonal perspective Atmospheric Chemistry and Physics. ,vol. 13, pp. 7053- 7074 ,(2013) , 10.5194/ACP-13-7053-2013
Xuejiao Deng, Xuexi Tie, Dui Wu, Xiuji Zhou, Xueyan Bi, Hanbo Tan, Fei Li, Chenglin Jiang, Long-term trend of visibility and its characterizations in the Pearl River Delta (PRD) region, China Atmospheric Environment. ,vol. 42, pp. 1424- 1435 ,(2008) , 10.1016/J.ATMOSENV.2007.11.025
David G. Streets, Carolyne Yu, Ye Wu, Mian Chin, Zongci Zhao, Tadahiro Hayasaka, Guangyu Shi, Aerosol trends over China, 1980–2000 Atmospheric Research. ,vol. 88, pp. 174- 182 ,(2008) , 10.1016/J.ATMOSRES.2007.10.016
Xuexi Tie, Sasha Madronich, Stacy Walters, David P Edwards, Paul Ginoux, Natalie Mahowald, RenYi Zhang, Chao Lou, Guy Brasseur, Assessment of the global impact of aerosols on tropospheric oxidants Journal of Geophysical Research. ,vol. 110, ,(2005) , 10.1029/2004JD005359
Qiang Zhang, Chunsheng Zhao, Xuexi Tie, Qiang Wei, Mengyu Huang, Guohui Li, Zhuming Ying, Chengcai Li, Characterizations of aerosols over the Beijing region: A case study of aircraft measurements Atmospheric Environment. ,vol. 40, pp. 4513- 4527 ,(2006) , 10.1016/J.ATMOSENV.2006.04.032
Jun-ji Cao, Qi-yuan Wang, Judith C. Chow, John G. Watson, Xue-xi Tie, Zhen-xing Shen, Ping Wang, Zhi-sheng An, Impacts of aerosol compositions on visibility impairment in Xi'an, China Atmospheric Environment. ,vol. 59, pp. 559- 566 ,(2012) , 10.1016/J.ATMOSENV.2012.05.036
Xuexi Tie, Junji Cao, Aerosol pollution in China: Present and future impact on environment Particuology. ,vol. 7, pp. 426- 431 ,(2009) , 10.1016/J.PARTIC.2009.09.003
G. Li, M. Zavala, W. Lei, A. P. Tsimpidi, V. A. Karydis, S. N. Pandis, M. R. Canagaratna, L. T. Molina, Simulations of organic aerosol concentrations in Mexico City using the WRF-CHEM model during the MCMA-2006/MILAGRO campaign Atmospheric Chemistry and Physics. ,vol. 11, pp. 3789- 3809 ,(2011) , 10.5194/ACP-11-3789-2011
Xuexi Tie, Sasha Madronich, Stacy Walters, Renyi Zhang, Phil Rasch, William Collins, Effect of clouds on photolysis and oxidants in the troposphere Journal of Geophysical Research. ,vol. 108, pp. 4642- ,(2003) , 10.1029/2003JD003659
Qiang Zhang, XinCheng Ma, Xuexi Tie, Mengyu Huang, Chunsheng Zhao, Vertical distributions of aerosols under different weather conditions: Analysis of in-situ aircraft measurements in Beijing, China Atmospheric Environment. ,vol. 43, pp. 5526- 5535 ,(2009) , 10.1016/J.ATMOSENV.2009.05.037