How a European network may help with estimating methane emissions on the French national scale

作者: Isabelle Pison , Antoine Berchet , Marielle Saunois , Philippe Bousquet , Grégoire Broquet

DOI: 10.5194/ACP-18-3779-2018

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摘要: Abstract. Methane emissions on the national scale in France 2012 are inferred by assimilating continuous atmospheric mixing ratio measurements from nine stations of European network ICOS located and surrounding countries. To assess robustness fluxes deduced our inversion system based an objectified quantification uncertainties, two complementary set-ups computed analysed: (i) a regional run correcting for spatial distribution (ii) a sectorial activity sectors scale. In addition, results compared with produced framework inter-comparison exercise InGOS project. The seasonal variability is consistent between different set-ups, maximum summer, likely due to agricultural activity. However, very high monthly posterior uncertainties (up ≈ 65 to 74 % May June) make it difficult attribute a specific sector. On yearly scales, inversions range 3835 4050 Gg CH4 3570 4190 Gg CH4 runs, respectively, consistently products. These estimates 25 to 55 % higher than total bottom-up approaches (biogeochemical models natural emissions, plus inventories anthropogenic ones), pointing at missing or underestimated sources and/or sources. More specifically, set-up, as 66% larger reported UNFCCC. Uncertainties annual budget 108 and 312 Gg CH4, i.e, 3 to 8 %, runs smaller available products, proving added value top-down inversions. Therefore, even though surface used in 2012 does not allow us fully constrain all regions accurately, set-up makes possible provide French methane uncertainty less 10 % timescale. Additional sites deployed since 2012 would help finer temporal scales attributing sectors.

参考文章(26)
Jean-Yves Dourmad, Jean Noblet, Daniel Sauvant, Maguy Eugène, Michel Vermorel, J Pierre Jouany, Evaluation quantitative des émissions de méthane entérique par les animaux d élevage en 2007 en France Productions Animales. ,vol. 21, pp. 403- 418 ,(2008)
A. L. Ganesan, A. J. Manning, A. Grant, D. Young, D .E. Oram, W. T. Sturges, J. B. Moncrieff, S. O'Doherty, Quantifying methane and nitrous oxide emissions from the UK and Ireland using a national-scale monitoring network Atmospheric Chemistry and Physics. ,vol. 15, pp. 6393- 6406 ,(2015) , 10.5194/ACP-15-6393-2015
R. L. Thompson, A. Stohl, L. X. Zhou, E. Dlugokencky, Y. Fukuyama, Y. Tohjima, S.-Y. Kim, H. Lee, E. G. Nisbet, R. E. Fisher, D. Lowry, R. F. Weiss, R. G. Prinn, S. O'Doherty, D. Young, J. W. C. White, Methane emissions in East Asia for 2000–2011 estimated using an atmospheric Bayesian inversion Journal of Geophysical Research. ,vol. 120, pp. 4352- 4369 ,(2015) , 10.1002/2014JD022394
L. Menut, B. Bessagnet, D. Khvorostyanov, M. Beekmann, N. Blond, A. Colette, I. Coll, G. Curci, G. Foret, A. Hodzic, S. Mailler, F. Meleux, J.-L. Monge, I. Pison, G. Siour, S. Turquety, M. Valari, R. Vautard, M. G. Vivanco, CHIMERE 2013: a model for regional atmospheric composition modelling Geoscientific Model Development. ,vol. 6, pp. 981- 1028 ,(2013) , 10.5194/GMD-6-981-2013
M. Darding, B. Lebègue, C. Kaiser, I. Xueref-Rémy, M. Ramonet, C. Yver Kwok, O. Laurent, A. Guemri, C. Philippon, B. Wastine, C. W. Rella, C. Vuillemin, F. Truong, M. Delmotte, V. Kazan, Comprehensive laboratory and field testing of cavity ring-down spectroscopy analyzers measuring H 2 O, CO 2 , CH 4 and CO Atmospheric Measurement Techniques. ,vol. 8, pp. 3867- 3892 ,(2015) , 10.5194/AMT-8-3867-2015
P. Bousquet, P. Ciais, J. B. Miller, E. J. Dlugokencky, D. A. Hauglustaine, C. Prigent, G. R. Van der Werf, P. Peylin, E.-G. Brunke, C. Carouge, R. L. Langenfelds, J. Lathière, F. Papa, M. Ramonet, M. Schmidt, L. P. Steele, S. C. Tyler, J. White, Contribution of anthropogenic and natural sources to atmospheric methane variability Nature. ,vol. 443, pp. 439- 443 ,(2006) , 10.1038/NATURE05132
J. L. Champeaux, V. Masson, F. Chauvin, ECOCLIMAP: a global database of land surface parameters at 1 km resolution Meteorological Applications. ,vol. 12, pp. 29- 32 ,(2005) , 10.1017/S1350482705001519
A. Berchet, I. Pison, F. Chevallier, P. Bousquet, J.-L. Bonne, J.-D. Paris, Objectified quantification of uncertainties in Bayesian atmospheric inversions Geoscientific Model Development. ,vol. 8, pp. 1525- 1546 ,(2015) , 10.5194/GMD-8-1525-2015
A. Berchet, I. Pison, F. Chevallier, J.-D. Paris, P. Bousquet, J.-L. Bonne, M. Y. Arshinov, B. D. Belan, C. Cressot, D. K. Davydov, E. J. Dlugokencky, A. V. Fofonov, A. Galanin, J. Lavrič, T. Machida, R. Parker, M. Sasakawa, R. Spahni, B. D. Stocker, J. Winderlich, Natural and anthropogenic methane fluxes in Eurasia: a mesoscale quantification by generalized atmospheric inversion Biogeosciences. ,vol. 12, pp. 5393- 5414 ,(2015) , 10.5194/BG-12-5393-2015
P. Bergamaschi, M. Corazza, U. Karstens, M. Athanassiadou, R. L. Thompson, I. Pison, A. J. Manning, P. Bousquet, A. Segers, A. T. Vermeulen, G. Janssens-Maenhout, M. Schmidt, M. Ramonet, F. Meinhardt, T. Aalto, L. Haszpra, J. Moncrieff, M. E. Popa, D. Lowry, M. Steinbacher, A. Jordan, S. O'Doherty, S. Piacentino, E. Dlugokencky, Top-down estimates of European CH4 and N2O emissions based on four different inverse models Atmospheric Chemistry and Physics. ,vol. 15, pp. 715- 736 ,(2015) , 10.5194/ACP-15-715-2015