Water-Soluble Ag Nanoclusters Exhibit Strong Two-Photon-Induced Fluorescence

作者: Sandeep A. Patel , Chris I. Richards , Jung-Cheng Hsiang , Robert M. Dickson

DOI: 10.1021/JA804710R

关键词:

摘要: Water-soluble ssDNA-encapsulated Ag clusters exhibit large two-photon cross sections reaching 50 000 GM, with high quantum yields in the red and near-IR. Three distinct, spectrally pure, several atom emitting at 660, 680, or 710 nm have been created rivaling those of much larger water-soluble semiconductor dots. Their stability, biocompatibility, small size offer promise nontoxic, sensitive high-resolution biological imaging.

参考文章(19)
Junhua Yu, Sandeep A. Patel, Robert M. Dickson, In Vitro and Intracellular Production of Peptide‐Encapsulated Fluorescent Silver Nanoclusters Angewandte Chemie. ,vol. 46, pp. 2028- 2030 ,(2007) , 10.1002/ANIE.200604253
Jeffrey T. Petty, Jie Zheng, Nicholas V. Hud, Robert M. Dickson, DNA-templated Ag nanocluster formation. Journal of the American Chemical Society. ,vol. 126, pp. 5207- 5212 ,(2004) , 10.1021/JA031931O
Johan Benesch, Agneta Askendal, Pentti Tengvall, The determination of thickness and surface mass density of mesothick immunoprecipitate layers by null ellipsometry and protein 125iodine labeling. Journal of Colloid and Interface Science. ,vol. 249, pp. 84- 90 ,(2002) , 10.1006/JCIS.2002.8247
C. Xu, W. Zipfel, J. B. Shear, R. M. Williams, W. W. Webb, Multiphoton fluorescence excitation: new spectral windows for biological nonlinear microscopy Proceedings of the National Academy of Sciences of the United States of America. ,vol. 93, pp. 10763- 10768 ,(1996) , 10.1073/PNAS.93.20.10763
Daniel R Larson, Warren R Zipfel, Rebecca M Williams, Stephen W Clark, Marcel P Bruchez, Frank W Wise, Watt W Webb, Water-Soluble Quantum Dots for Multiphoton Fluorescence Imaging in Vivo Science. ,vol. 300, pp. 1434- 1436 ,(2003) , 10.1126/SCIENCE.1083780
Marius A. Albota, Chris Xu, Watt W. Webb, Two-photon fluorescence excitation cross sections of biomolecular probes from 690 to 960 nm Applied Optics. ,vol. 37, pp. 7352- 7356 ,(1998) , 10.1364/AO.37.007352
Chris I. Richards, Sungmoon Choi, Jung-Cheng Hsiang, Yasuko Antoku, Tom Vosch, Angelo Bongiorno, Yih-Ling Tzeng, Robert M. Dickson, Oligonucleotide-stabilized Ag nanocluster fluorophores. Journal of the American Chemical Society. ,vol. 130, pp. 5038- 5039 ,(2008) , 10.1021/JA8005644
J. Tiggesbäumker, L. Köller, H.O. Lutz, K.H. Meiwes-Broer, Giant resonances in silver-cluster photofragmentation Chemical Physics Letters. ,vol. 190, pp. 42- 47 ,(1992) , 10.1016/0009-2614(92)86099-4
Joanna Lukomska, Ignacy Gryczynski, Joanna Malicka, Slawomir Makowiec, Joseph R. Lakowicz, Zygmunt Gryczynski, Two-photon induced fluorescence of Cy5-DNA in buffer solution and on silver island films Biochemical and Biophysical Research Communications. ,vol. 328, pp. 78- 84 ,(2005) , 10.1016/J.BBRC.2004.12.148
Mark G. Kuzyk, Fundamental limits on two-photon absorption cross sections Journal of Chemical Physics. ,vol. 119, pp. 8327- 8334 ,(2003) , 10.1063/1.1611474