Quantum diffusion wave-function approach to two-dimensional vibronic spectroscopy
作者： Johannes Wehner , Mirjam Falge , Walter T. Strunz , Volker Engel
DOI: 10.1063/1.4896705
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摘要: We apply the quantum diffusion wavefunction approach to calculate vibronic two-dimensional (2D) spectra. As an example, we use a system consisting of two electronic states with harmonic oscillator potentials which are coupled bath and interact three time-delayed laser pulses. The first- second-order perturbative wave functions enter into expression for third-order polarization determined sufficient number stochastic runs. wave-packet approach, besides being alternative technique spectra, offers intuitive insight dissipation dynamics its relation 2D
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Joel Yuen-Zhou, Alán Aspuru-Guzik, Jacob J. Krich, A witness for coherent electronic vs vibronic-only oscillations in ultrafast spectroscopy Journal of Chemical Physics. ,vol. 136, pp. 234501- 234501 ,(2012) , 10.1063/1.4725498
John D. Hybl, Allison W. Albrecht, Sarah M. Gallagher Faeder, David M. Jonas, Two-dimensional electronic spectroscopy Chemical Physics Letters. ,vol. 297, pp. 307- 313 ,(1998) , 10.1016/S0009-2614(98)01140-3
Joachim Seibt, Klaus Renziehausen, Dmitri V. Voronine, Volker Engel, Probing the geometry dependence of molecular dimers with two-dimensional-vibronic spectroscopy Journal of Chemical Physics. ,vol. 130, pp. 134318- 134318 ,(2009) , 10.1063/1.3086935
Stefan Ruetzel, Meike Diekmann, Patrick Nuernberger, Christof Walter, Bernd Engels, Tobias Brixner, Multidimensional spectroscopy of photoreactivity Proceedings of the National Academy of Sciences of the United States of America. ,vol. 111, pp. 4764- 4769 ,(2014) , 10.1073/PNAS.1323792111
Minhaeng Cho, Graham R. Fleming, The integrated photon echo and solvation dynamics. II. Peak shifts and two- dimensional photon echo of a coupled chromophore system Journal of Chemical Physics. ,vol. 123, pp. 114506- 114506 ,(2005) , 10.1063/1.1955444
Jens Bredenbeck, Jan Helbing, Christoph Kolano, Peter Hamm, Ultrafast 2D–IR Spectroscopy of Transient Species ChemPhysChem. ,vol. 8, pp. 1747- 1756 ,(2007) , 10.1002/CPHC.200700148
Leah Z. Sharp, Dassia Egorova, Towards microscopic assignment of oscillative signatures in two-dimensional electronic photon-echo signals of vibronic oligomers: a vibronic dimer model. Journal of Chemical Physics. ,vol. 139, pp. 144304- 144304 ,(2013) , 10.1063/1.4822425
Martin Schlesinger, Marcel Mudrich, Frank Stienkemeier, Walter T. Strunz, Dissipative vibrational wave packet dynamics of alkali dimers attached to helium nanodroplets Chemical Physics Letters. ,vol. 490, pp. 245- 248 ,(2010) , 10.1016/J.CPLETT.2010.03.060
Sarah M. Gallagher Faeder, David M. Jonas, Two-Dimensional Electronic Correlation and Relaxation Spectra: Theory and Model Calculations Journal of Physical Chemistry A. ,vol. 103, pp. 10489- 10505 ,(1999) , 10.1021/JP9925738
Klaus Renziehausen, Philipp Marquetand, Volker Engel, On the divergence of time-dependent perturbation theory applied to laser-induced molecular transitions Journal of Physics B. ,vol. 42, pp. 195402- ,(2009) , 10.1088/0953-4075/42/19/195402