Improving the pollutant removal efficiency of packed-bed plasma reactors incorporating ferroelectric components

作者: Ana Gómez-Ramírez , Antonio M. Montoro-Damas , Miguel A. Rodríguez , Agustín R. González-Elipe , José Cotrino

DOI: 10.1016/J.CEJ.2016.11.065

关键词:

摘要: Abstract In this work we have studied the plasma removal of air contaminants such as methane, chloroform, toluene and acetone in two parallel plate packed-bed dielectric barrier discharge (DBD) reactors different sizes. Removal energy efficiencies been determined a function residence time contaminated within reactor, kind material (ferroelectrics or classical materials), frequency incorporation ferroelectric onto active electrode together with inter-electrode pellets filling gap. Results at low small reactor showed an enhancement efficiency (e.g., it was multiplied by factor six three for respectively) yield increased from 22% to 52% chloroform 15% 21% methane). Such enhancements attributed higher electrons lower capacitance found plate-modified configuration. A careful analysis reaction electron distributions investigated conditions simulation electric field necks between ferroelectric/dielectric complete present study. Overall, obtained results prove critical role architecture operating enhanced performance pollution processes using DBD systems.

参考文章(58)
Atsushi Ogata, Koichi Mizuno, Satoshi Kushiyama, Toshiaki Yamamoto, METHANE DECOMPOSITION IN A BARIUM TITANATE PACKED-BED NONTHERMAL PLASMA REACTOR Plasma Chemistry and Plasma Processing. ,vol. 18, pp. 363- 373 ,(1998) , 10.1023/A:1021897419040
Takao Matsumoto, Douyan Wang, Takao Namihira, Hidenori Akiyam, Non-Thermal Plasma Technic for Air Pollution Control InTech. ,(2012) , 10.5772/50419
Ulrich Kogelschatz, Dielectric-barrier Discharges: Their History, Discharge Physics, and Industrial Applications Plasma Chemistry and Plasma Processing. ,vol. 23, pp. 1- 46 ,(2003) , 10.1023/A:1022470901385
A.M. Montoro-Damas, J. Javier Brey, Miguel A. Rodríguez, Agustín R. González-Elipe, José Cotrino, Plasma reforming of methane in a tunable ferroelectric packed-bed dielectric barrier discharge reactor Journal of Power Sources. ,vol. 296, pp. 268- 275 ,(2015) , 10.1016/J.JPOWSOUR.2015.07.038
Liying Jiang, Runye Zhu, Yubo Mao, Jianmeng Chen, Liang Zhang, Conversion characteristics and production evaluation of styrene/o-xylene mixtures removed by DBD pretreatment. International Journal of Environmental Research and Public Health. ,vol. 12, pp. 1334- 1350 ,(2015) , 10.3390/IJERPH120201334
F. Holzer, F. D. Kopinke, U. Roland, Influence of Ferroelectric Materials and Catalysts on the Performance of Non-Thermal Plasma (NTP) for the Removal of Air Pollutants Plasma Chemistry and Plasma Processing. ,vol. 25, pp. 595- 611 ,(2005) , 10.1007/S11090-005-6804-1
Alice M. Harling, David J. Glover, J. Christopher Whitehead, Kui Zhang, Industrial Scale Destruction of Environmental Pollutants using a Novel Plasma Reactor Industrial & Engineering Chemistry Research. ,vol. 47, pp. 5856- 5860 ,(2008) , 10.1021/IE8001364
J G Eden, S-J Park, N P Ostrom, S T McCain, C J Wagner, B A Vojak, J Chen, C Liu, P von Allmen, F Zenhausern, D J Sadler, C Jensen, D L Wilcox, J J Ewing, Microplasma devices fabricated in silicon, ceramic, and metal/polymer structures: Arrays, emitters and photodetectors Journal of Physics D. ,vol. 36, pp. 2869- 2877 ,(2003) , 10.1088/0022-3727/36/23/001