Advancing Model Systems for Fundamental Laboratory Studies of Sea Spray Aerosol Using the Microbial Loop

作者: Christopher Lee , Camille M. Sultana , Douglas B. Collins , Mitchell V. Santander , Jessica L. Axson

DOI: 10.1021/ACS.JPCA.5B03488

关键词:

摘要: Sea spray aerosol (SSA) particles represent one of the most abundant surfaces available for heterogeneous reactions to occur upon and thus profoundly alter composition troposphere. In an effort better understand tropospheric reaction processes, fundamental laboratory studies must be able accurately reproduce chemical complexity SSA. Here we describe a new approach that uses microbial processes control seawater SSA particle composition. By inducing phytoplankton bloom, are create dynamic ecosystem interactions between marine microorganisms, which serve organic mixtures present in seawater. Using this controlled approach, changes become reflected 4 10 d after peak chlorophyll-a. This producing varying dominant provides foundation further investigations physical...

参考文章(88)
J. P. D. Abbatt, M. J. Molina, Heterogeneous interactions of nitryl hypochlorite and hydrogen chloride on nitric acid trihydrate at 202 K The Journal of Physical Chemistry. ,vol. 96, pp. 7674- 7679 ,(1992) , 10.1021/J100198A036
Kostas Tsigaridis, Dorothy Koch, Surabi Menon, Uncertainties and importance of sea spray composition on aerosol direct and indirect effects Journal of Geophysical Research. ,vol. 118, pp. 220- 235 ,(2013) , 10.1029/2012JD018165
Matteo Rinaldi, Sandro Fuzzi, Stefano Decesari, Salvatore Marullo, Rosalia Santoleri, Antonello Provenzale, Jost von Hardenberg, Darius Ceburnis, Aditya Vaishya, Colin D. O'Dowd, Maria Cristina Facchini, Is chlorophyll‐a the best surrogate for organic matter enrichment in submicron primary marine aerosol? Journal of Geophysical Research. ,vol. 118, pp. 4964- 4973 ,(2013) , 10.1002/JGRD.50417
Michael Cunliffe, Robert C. Upstill-Goddard, J. Colin Murrell, Microbiology of aquatic surface microlayers. Fems Microbiology Reviews. ,vol. 35, pp. 233- 246 ,(2011) , 10.1111/J.1574-6976.2010.00246.X
Cassandra J. Gaston, Hiroshi Furutani, Sergio A. Guazzotti, Keith R. Coffee, Timothy S. Bates, Patricia K. Quinn, Lihini I. Aluwihare, B. Gregory Mitchell, Kimberly A. Prather, Unique ocean-derived particles serve as a proxy for changes in ocean chemistry Journal of Geophysical Research. ,vol. 116, ,(2011) , 10.1029/2010JD015289
Yuan You, Mackenzie L. Smith, Mijung Song, Scot T. Martin, Allan K. Bertram, Liquid–liquid phase separation in atmospherically relevant particles consisting of organic species and inorganic salts International Reviews in Physical Chemistry. ,vol. 33, pp. 43- 77 ,(2014) , 10.1080/0144235X.2014.890786
D. F. Bird, J. Kalff, Empirical relationships between bacterial abundance and chlorophyll concentration in fresh and marine waters Canadian Journal of Fisheries and Aquatic Sciences. ,vol. 41, pp. 1015- 1023 ,(1984) , 10.1139/F84-118
David C. Smith, Grieg F. Steward, Richard A. Long, Farooq Azam, Bacterial mediation of carbon fluxes during a diatom bloom in a mesocosm Deep Sea Research Part II: Topical Studies in Oceanography. ,vol. 42, pp. 75- 97 ,(1995) , 10.1016/0967-0645(95)00005-B
M Gilstad, E Sakshaug, Growth rates of ten diatom species from the Barents Sea at different irradiances and day lengths Marine Ecology Progress Series. ,vol. 64, pp. 169- 173 ,(1990) , 10.3354/MEPS064169
Marc Bouvet, Nicolas Hoepffner, Mark D. Dowell, Parameterization of a spectral solar irradiance model for the global ocean using multiple satellite sensors Journal of Geophysical Research: Oceans. ,vol. 107, pp. 8- 1 ,(2002) , 10.1029/2001JC001126