Present and future trends in the atmospheric burden of ozone-depleting halogens

作者: S. A. Montzka , J. H. Butler , J.W. Elkins , T. M. Thompson , A. D. Clarke

DOI: 10.1038/19499

关键词:

摘要: The burden of ozone-depleting chemicals in the lower atmosphere has been decreasing since 1994 as a result Montreal Protocol1,3. Here we show how individual have influenced this decline, order to estimate could change near future. Our measurements atmospheric concentrations persistent, anthropogenic that account for most halogens today's stratosphere decline stems predominantly from decrease load trichloroethane (CH3CCl3), previously common cleaning solvent. influence chemical on now peaked, however, and will become much smaller over next five ten years. As lessens, theburden halogen be sustained only if emissions other halocarbons fall. Although gases regulated by Protocol decreased substantially past years (refs 4), potent gas CBrClF2 (halon-1211) remained fairly constant during period12,29, despite stringent limits production developed countries 1994. consequent accumulation halon is retarding more than any persistent gas.

参考文章(25)
B. A. Callander, L. G. Meira Filho, John Theodore Houghton, K. Maskell, A. Kattenberg, N. Harris, Climate Change 1995: The Science of Climate Change ,(1996)
James B. Burkholder, Robert R. Wilson, Tomasz Gierczak, Ranajit Talukdar, Stuart A. McKeen, John J. Orlando, Ghanshyam L. Vaghjiani, A. R. Ravishankara, Atmospheric fate of CF3Br, CF2Br2, CF2ClBr, and CF2BrCF2BR Journal of Geophysical Research. ,vol. 96, pp. 5025- 5043 ,(1991) , 10.1029/90JD02735
Drew T. Shindell, David Rind, Patrick Lonergan, Increased polar stratospheric ozone losses and delayed eventual recovery owing to increasing greenhouse-gas concentrations Nature. ,vol. 392, pp. 589- 592 ,(1998) , 10.1038/33385
D. Fisher, M.K.W. Ko, P. Fraser, S.A. Penkett, J.A. Kaye, S.P. Sander, P. Bloomfield, F.M. Ormond, Report on concentrations, lifetimes, and trends of CFCs, halons, and related species Unknow. ,(1994)
S. A. Montzka, R. C. Myers, J. H. Butler, J. W. Elkins, S. O. Cummings, Global tropospheric distribution and calibration scale of HCFC-22 Geophysical Research Letters. ,vol. 20, pp. 703- 706 ,(1993) , 10.1029/93GL00753
C. M. Volk, J. W. Elkins, D. W. Fahey, G. S. Dutton, J. M. Gilligan, M. Loewenstein, J. R. Podolske, K. R. Chan, M. R. Gunson, Evaluation of source gas lifetimes from stratospheric observations Journal of Geophysical Research. ,vol. 102, pp. 25543- 25564 ,(1997) , 10.1029/97JD02215
J. W. Elkins, T. M. Thompson, T. H. Swanson, J. H. Butler, B. D. Hall, S. O. Cummings, D. A. Fishers, A. G. Raffo, Decrease in the growth rates of atmospheric chlorofluorocarbons 11 and 12 Nature. ,vol. 364, pp. 780- 783 ,(1993) , 10.1038/364780A0
Charles H. Jackman, Eric L. Fleming, Sushil Chandra, David B. Considine, Joan E. Rosenfield, Past, present, and future modeled ozone trends with comparisons to observed trends Journal of Geophysical Research. ,vol. 101, pp. 28753- 28767 ,(1996) , 10.1029/96JD03088
P. Fraser, D. Cunnold, F. Alyea, R. Weiss, R. Prinn, P. Simmonds, B. Miller, R. Langenfelds, Lifetime and emission estimates of 1,1,2-trichlorotrifluorethane (CFC-113) from daily global background observations June 1982-June 1994 Journal of Geophysical Research: Atmospheres. ,vol. 101, pp. 12585- 12599 ,(1996) , 10.1029/96JD00574
James H. Butler, Stephen A. Montzka, Andrew D. Clarke, Jürgen M. Lobert, James W. Elkins, Growth and distribution of halons in the atmosphere Journal of Geophysical Research. ,vol. 103, pp. 1503- 1511 ,(1998) , 10.1029/97JD02853