Synthesis of core-shell UiO-66-poly(m-phenylenediamine) composites for removal of hexavalent chromium.
作者： Haiying Wang , Lanjing Hou , Yujun Shen , Lei Huang , Yingjie He
DOI: 10.1007/S11356-019-07070-1
关键词:
摘要: The present research developed a direct in situ heterogeneous method to synthesize UiO-66-poly(m-phenylenediamine) core-shell nanostructures by inducing assembly of m-phenylenediamine radical on UiO-66 surfaces. strong interaction between negative charged and positive from the oxidation monomer is major driving force. produced composites exhibited distinct morphology with controllable surface features. UiO-661-PmPD0.5 showed uniform PmPD shell thickness 40–60 nm nanocomposite high specific area 319.77 m2 g−1. Moreover, Cr(VI) adsorption amount polymeric nanocomposites can reach as 745 mg g−1, far beyond performance original PmPD. tends be equilibrium within 300 min. This opens hopeful window for facile large-scale fabrication configuration, exhibiting prospect heavy metal removal water.
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sci-hub.se 参考文章(48)
Mohammadtaghi Vakili, Mohd Rafatullah, Mahamad Hakimi Ibrahim, Ahmad Zuhairi Abdullah, Babak Salamatinia, Zahra Gholami, Oil Palm Biomass as an Adsorbent for Heavy Metals Reviews of Environmental Contamination and Toxicology. ,vol. 232, pp. 61- 88 ,(2014) , 10.1007/978-3-319-06746-9_3
Ahmet Kaya, Canan Onac, H. Korkmaz Alpoguz, Aydan Yilmaz, Necip Atar, Removal of Cr(VI) through calixarene based polymer inclusion membrane from chrome plating bath water Chemical Engineering Journal. ,vol. 283, pp. 141- 149 ,(2016) , 10.1016/J.CEJ.2015.07.052
Kuang He, Yuancai Chen, Zhenghua Tang, Yongyou Hu, Removal of heavy metal ions from aqueous solution by zeolite synthesized from fly ash. Environmental Science and Pollution Research. ,vol. 23, pp. 2778- 2788 ,(2016) , 10.1007/S11356-015-5422-6
Xin-Gui Li, Mei-Rong Huang, Wei Duan, Yu-Liang Yang, Novel multifunctional polymers from aromatic diamines by oxidative polymerizations. Chemical Reviews. ,vol. 102, pp. 2925- 3030 ,(2002) , 10.1021/CR010423Z
Yafeng Li, Yan Liu, Wenyuan Gao, Limei Zhang, Wei Liu, Jingjing Lu, Zhen Wang, Yun-Jiao Deng, None, Microwave-assisted synthesis of UIO-66 and its adsorption performance towards dyes CrystEngComm. ,vol. 16, pp. 7037- 7042 ,(2014) , 10.1039/C4CE00526K
Weizhen Liu, Feng Huang, YongJing Wang, Ting Zou, Jinsheng Zheng, Zhang Lin, Recycling Mg(OH)2 Nanoadsorbent during Treating the Low Concentration of CrVI Environmental Science & Technology. ,vol. 45, pp. 1955- 1961 ,(2011) , 10.1021/ES1035199
Saeid Azizian, Comment on “Kinetics of Solute Adsorption at Solid/Solution Interfaces: A Theoretical Development of the Empirical Pseudo-First and Pseudo-Second Order Kinetic Rate Equations, Based on Applying the Statistical Rate Theory of Interfacial Transport” The Journal of Physical Chemistry B. ,vol. 111, pp. 318- 318 ,(2007) , 10.1021/JP065024S
Zhen Su, Liyuan Zhang, Liyuan Chai, Wanting Yu, Haiying Wang, Yu Shi, Methanol-induced formation of 1D poly(m-phenylenediamine) by conventional chemical oxidative polymerization exhibiting superior Ag+ adsorption ability RSC Advances. ,vol. 3, pp. 8660- 8665 ,(2013) , 10.1039/C3RA41568F
K.Y. Foo, B.H. Hameed, Insights into the modeling of adsorption isotherm systems Chemical Engineering Journal. ,vol. 156, pp. 2- 10 ,(2010) , 10.1016/J.CEJ.2009.09.013
Jasmina Hafizovic Cavka, Søren Jakobsen, Unni Olsbye, Nathalie Guillou, Carlo Lamberti, Silvia Bordiga, Karl Petter Lillerud, A new zirconium inorganic building brick forming metal organic frameworks with exceptional stability. Journal of the American Chemical Society. ,vol. 130, pp. 13850- 13851 ,(2008) , 10.1021/JA8057953