New-particle formation, growth and climate-relevant particle production in Egbert, Canada: analysis from 1 year of size-distribution observations

作者: J. R. Pierce , D. M. Westervelt , S. A. Atwood , E. A. Barnes , W. R. Leaitch

DOI: 10.5194/ACP-14-8647-2014

关键词:

摘要: Abstract. Aerosol particle nucleation, or new-particle formation, is the dominant contributor to number in atmosphere. However, these particles must grow through condensation of low-volatility vapors without coagulating with larger, preexisting order reach climate-relevant sizes (diameters larger than 50–100 nm), where may affect clouds and radiation. In this paper, we use 1 year size-distribution measurements from Egbert, Ontario, Canada calculate frequency regional-scale new-particle-formation events, rates, growth rates fraction new that survive sizes. Regional-scale events occur on 14–31% days (depending stringency classification criteria), event peaking spring fall. New-particle-formation are similar those measured at other midlatitude continental sites. We roughly half (with diameters nm) Egbert formed events. With addition meteorological SO2 measurements, find formation often occurs under synoptic conditions associated high surface pressure large-scale subsidence cause sunny clean-air flow north west. also when air flows polluted regions south southwest Egbert. The tend be faster during south/southwest conditions.

参考文章(45)
Nicola Stuber, D. Oram, David W. Fahey, Gunnar Myhre, D. Etheridge, Karen Rosenlof, James Haywood, Ulrike Lohmann, Judith Lean, Michael Ponater, S.K. Solanki, Piers Forster, R. Weiss, Michael Schulz, Ronald Prinn, J.W. Elkins, Robert Sausen, Graciela Raga, Terje Berntsen, T. Takemura, A.C. Manning, P. Fraser, Venkatachalam Ramaswamy, E. Dlugokencky, W.D. Collins, Greg Bodeker, S. Montzka, David Rind, John Nganga, S. Piper, Christiane Textor, David C. Lowe, Garry Stenchikov, Marvyn Geller, G. Reid, K. O'Shaughnessy, Rob van Dorland, K. Lassey, D. Schwarzkopf, P. Foukal, T.J. Conway, T. Whorf, Oliver Boucher, R. Wang, Richard Betts, Paulo Artaxo, G.-K. Plattner, Stefan Kinne, N. Ramankutty, C.D. Keeling, F. Joos, Changes in Atmospheric Constituents and in Radiative Forcing Climate Change 2007 : The Physical Science Basis, Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change. ,vol. 141, pp. 129- 234 ,(2007)
N. M. Donahue, E. R. Trump, J. R. Pierce, I. Riipinen, Theoretical constraints on pure vapor‐pressure driven condensation of organics to ultrafine particles Geophysical Research Letters. ,vol. 38, ,(2011) , 10.1029/2011GL048115
P. Crippa, S.C. Pryor, Spatial and temporal scales of new particle formation events in eastern North America Atmospheric Environment. ,vol. 75, pp. 257- 264 ,(2013) , 10.1016/J.ATMOSENV.2013.04.051
W. Richard Leaitch, Anne Marie Macdonald, Peter C. Brickell, John Liggio, Steve J. Sjostedt, Alexander Vlasenko, Jan W. Bottenheim, Lin Huang, Shao-Meng Li, Peter S.K. Liu, Desiree Toom-Sauntry, Katherine A. Hayden, Sangeeta Sharma, Nicole C. Shantz, H. Allan Wiebe, Wendy Zhang, Jonathan P.D. Abbatt, Jay G. Slowik, Rachel Y.-W. Chang, Lynn M. Russell, Rachel E. Schwartz, Satoshi Takahama, John T. Jayne, Nga Lee Ng, Temperature response of the submicron organic aerosol from temperate forests Atmospheric Environment. ,vol. 45, pp. 6696- 6704 ,(2011) , 10.1016/J.ATMOSENV.2011.08.047
R. J. CHARLSON, S. E. SCHWARTZ, J. M. HALES, R. D. CESS, J. A. COAKLEY, J. E. HANSEN, D. J. HOFMANN, Climate Forcing by Anthropogenic Aerosols Science. ,vol. 255, pp. 423- 430 ,(1992) , 10.1126/SCIENCE.255.5043.423
C. Kuang, P. H. McMurry, A. V. McCormick, Determination of cloud condensation nuclei production from measured new particle formation events Geophysical Research Letters. ,vol. 36, ,(2009) , 10.1029/2009GL037584
Hanna Vehkamäki, Markku Kulmala, Ismo Napari, Kari EJ Lehtinen, Claudia Timmreck, Madis Noppel, Ari Laaksonen, An improved parameterization for sulfuric acid–water nucleation rates for tropospheric and stratospheric conditions Journal of Geophysical Research. ,vol. 107, pp. 4622- ,(2002) , 10.1029/2002JD002184
Fangqun Yu, Diurnal and Seasonal Variations of Ultrafine Particle Formation in Anthropogenic SO2 Plumes Environmental Science & Technology. ,vol. 44, pp. 2011- 2015 ,(2010) , 10.1021/ES903228A
Ilona Riipinen, Taina Yli-Juuti, Jeffrey R. Pierce, Tuukka Petäjä, Douglas R. Worsnop, Markku Kulmala, Neil M. Donahue, The contribution of organics to atmospheric nanoparticle growth Nature Geoscience. ,vol. 5, pp. 453- 458 ,(2012) , 10.1038/NGEO1499
Mikael Ehn, Joel A. Thornton, Einhard Kleist, Mikko Sipilä, Heikki Junninen, Iida Pullinen, Monika Springer, Florian Rubach, Ralf Tillmann, Ben Lee, Felipe Lopez-Hilfiker, Stefanie Andres, Ismail-Hakki Acir, Matti Rissanen, Tuija Jokinen, Siegfried Schobesberger, Juha Kangasluoma, Jenni Kontkanen, Tuomo Nieminen, Theo Kurtén, Lasse B. Nielsen, Solvejg Jørgensen, Henrik G. Kjaergaard, Manjula Canagaratna, Miikka Dal Maso, Torsten Berndt, Tuukka Petäjä, Andreas Wahner, Veli-Matti Kerminen, Markku Kulmala, Douglas R. Worsnop, Jürgen Wildt, Thomas F. Mentel, A large source of low-volatility secondary organic aerosol Nature. ,vol. 506, pp. 476- 479 ,(2014) , 10.1038/NATURE13032