Shipborne observations reveal contrasting Arctic marine, Arctic terrestrial and Pacific marine aerosol properties

作者: Jiyeon Park , Manuel Dall'Osto , Kihong Park , Yeontae Gim , Hyo Jin Kang

DOI: 10.5194/ACP-20-5573-2020

关键词:

摘要: Abstract. There are few shipborne observations addressing the factors influencing the relationships of formation and growth aerosol particles with cloud condensation nuclei (CCN) in remote marine environments. In this study, the physical properties throughout Arctic Ocean and Pacific were measured aboard Korean icebreaker R/V Araon during the summer 2017 for 25 d. A number new particle (NPF) events frequently observed both terrestrial and Arctic air masses. By striking contrast, NPF events not detected in Pacific Three major categories therefore discussed: (1)  (aerosol concentration CN 2.5 : 413±442  cm −3 ), (2) Arctic (CN 1622±1450 ) (3) Pacific 397±185 following mass back-trajectory analysis. conclusion of study is only that a source of secondary relative to but also that open-ocean sympagic terrestrially influenced coastal ecosystems both contribute shaping size distributions. We suggest terrestrial ecosystems – including river outflows tundra strongly affect aerosol emissions areas, possibly more than anthropogenic Arctic emissions. The increased discharge, emissions and melting sea ice should be considered future atmospheric composition climate simulations. average CCN concentrations at a supersaturation ratios 0.4 % 35±40 , 71±47 204±87 marine, Arctic terrestrial categories, respectively. Our results aim help evaluate how anthropogenic natural atmospheric sources processes composition cloud properties.

参考文章(101)
Raluca Ciuraru, Ludovic Fine, Manuela van Pinxteren, Barbara D’Anna, Hartmut Herrmann, Christian George, Photosensitized production of functionalized and unsaturated organic compounds at the air-sea interface. Scientific Reports. ,vol. 5, pp. 12741- 12741 ,(2015) , 10.1038/SREP12741
I. A. Shiklomanov, A. I. Shiklomanov, R. B. Lammers, B. J. Peterson, C. J. Vorosmarty, THE DYNAMICS OF RIVER WATER INFLOW TO THE ARCTIC OCEAN Springer Netherlands. pp. 281- 296 ,(2000) , 10.1007/978-94-011-4132-1_13
Betty Croft, Randall V. Martin, W. Richard Leaitch, Peter Tunved, Thomas J. Breider, Stephen D. D'Andrea, Jeffrey R. Pierce, Processes controlling the annual cycle of Arctic aerosol number and size distributions Atmospheric Chemistry and Physics. ,vol. 16, pp. 3665- 3682 ,(2016) , 10.5194/ACP-16-3665-2016
K. S. Law, A. Stohl, Arctic air pollution : Origins and impacts Science. ,vol. 315, pp. 1537- 1540 ,(2007) , 10.1126/SCIENCE.1137695
Patrick Faubert, Päivi Tiiva, Åsmund Rinnan, Anders Michelsen, Jarmo K. Holopainen, Riikka Rinnan, Doubled volatile organic compound emissions from subarctic tundra under simulated climate warming New Phytologist. ,vol. 187, pp. 199- 208 ,(2010) , 10.1111/J.1469-8137.2010.03270.X
S. Twomey, Pollution and the Planetary Albedo Atmospheric Environment. ,vol. 41, pp. 1251- 1256 ,(1974) , 10.1016/0004-6981(74)90004-3
Seong Soo Yum, James G. Hudson, Yonghong Xie, Comparisons of cloud microphysics with cloud condensation nuclei spectra over the summertime Southern Ocean Journal of Geophysical Research. ,vol. 103, pp. 16625- 16636 ,(1998) , 10.1029/98JD01513
Josep Peñuelas, Michael Staudt, BVOCs and global change Trends in Plant Science. ,vol. 15, pp. 133- 144 ,(2010) , 10.1016/J.TPLANTS.2009.12.005
M. J. Potosnak, B. M. Baker, L. LeStourgeon, S. M. Disher, K. L. Griffin, M. S. Bret-Harte, G. Starr, Isoprene emissions from a tundra ecosystem Biogeosciences. ,vol. 10, pp. 871- 889 ,(2013) , 10.5194/BG-10-871-2013
Michelle Schollert, Sebrina Burchard, Patrick Faubert, Anders Michelsen, Riikka Rinnan, Biogenic volatile organic compound emissions in four vegetation types in high arctic Greenland Polar Biology. ,vol. 37, pp. 237- 249 ,(2014) , 10.1007/S00300-013-1427-0