The dominant mechanism of the explosive rise of PM2.5 after significant pollution emissions reduction in Beijing from 2017 to the COVID-19 pandemic in 2020

作者: Tian Zhang , Huizheng Che , Zhiqiang Gong , Yaqiang Wang , Jizhi Wang

DOI: 10.1016/J.APR.2020.11.008

关键词:

摘要: Abstract The Chinese government implemented strict emission reduction measures of air pollution between 2013 and 2017. However, from the winter 2017 until February 2020, during COVID-19 pandemic, twenty explosive rise (ER) events PM2.5 mass in twelve heavy aerosol episodes (HPEs) still appeared Beijing its vicinity (BIV). To explore controlling mechanism for ER under condition drastically reduced emissions, vertical structure meteorological elements by L-band second-level sounding properties Lidar were investigated associating with analysis surface concentration mass, main precursor gases, as well black carbon (BC) seven-wavelength Aethalometer. planetary boundary layer height (BLH) was also estimated together an unfavorable index (PLAM) that can quantify impact conditions to cause change concentration. results suggested reoccurrence's fundamental is emissions have not yet fallen sufficiently a level decouple HPEs conditions. During period, BLH dropped significantly. fact PM2.5, increased almost similar proportion, indicating caused accumulation dominant reason phenomenon compared chemical conversion factor. two-way feedback effect further worsened typically interpreted 54%–93% ER. An HPE starting 8 Feb. 2020 period underwent one worst conditions, quantified PLAM, BIV since 2013. average only about 66% 2016. It shows substantial reduces primarily before when facing equivalent These combined suggest China's continuous efforts reduce proceed right direction achieved desired results.

参考文章(31)
Qiang Zhang, Kebin He, Hong Huo, Policy: Cleaning China's air Nature. ,vol. 484, pp. 161- 162 ,(2012) , 10.1038/484161A
X. Y. Zhang, Y. Q. Wang, X. C. Zhang, W. Guo, T. Niu, S. L. Gong, Y. Yin, P. Zhao, J. L. Jin, M. Yu, Aerosol monitoring at multiple locations in China: contributions of EC and dust to aerosol light absorption Tellus B. ,vol. 60, pp. 647- 656 ,(2008) , 10.1111/J.1600-0889.2008.00359.X
J. Z. Wang, S. L. Gong, X. Y. Zhang, Y. Q. Yang, Q. Hou, C. H. Zhou, Y. Q. Wang, A Parameterized Method for Air-Quality Diagnosis and Its Applications Advances in Meteorology. ,vol. 2012, pp. 1- 10 ,(2012) , 10.1155/2012/238589
XY Zhang, YQ Wang, WL Lin, YM Zhang, XC Zhang, S Gong, P Zhao, YQ Yang, JZ Wang, Q Hou, XL Zhang, HZ Che, JP Guo, Y Li, None, CHANGES OF ATMOSPHERIC COMPOSITION AND OPTICAL PROPERTIES OVER BEIJING—2008 Olympic Monitoring Campaign Bulletin of the American Meteorological Society. ,vol. 90, pp. 1633- 1651 ,(2009) , 10.1175/2009BAMS2804.1
Jizhi Wang, Yaqiang Wang, Hua Liu, Yuanqin Yang, Xiaoye Zhang, Yi Li, Yangmei Zhang, Guo Deng, Diagnostic identification of the impact of meteorological conditions on PM2.5 concentrations in Beijing Atmospheric Environment. ,vol. 81, pp. 158- 165 ,(2013) , 10.1016/J.ATMOSENV.2013.08.033
Song Guo, Min Hu, Misti L. Zamora, Jianfei Peng, Dongjie Shang, Jing Zheng, Zhuofei Du, Zhijun Wu, Min Shao, Limin Zeng, Mario J. Molina, Renyi Zhang, Elucidating severe urban haze formation in China Proceedings of the National Academy of Sciences of the United States of America. ,vol. 111, pp. 17373- 17378 ,(2014) , 10.1073/PNAS.1419604111
B. Zheng, Q. Zhang, Y. Zhang, K. B. He, K. Wang, G. J. Zheng, F. K. Duan, Y. L. Ma, T. Kimoto, Heterogeneous chemistry: a mechanism missing in current models to explain secondary inorganic aerosol formation during the January 2013 haze episode in North China Atmospheric Chemistry and Physics. ,vol. 15, pp. 2031- 2049 ,(2015) , 10.5194/ACP-15-2031-2015
YuanQin YANG, JianNong QUAN, YaQiang WANG, YangMei ZHANG, GuoLiang CAO, Qiang ZHANG, WeiGang WANG, JiZhi WANG, JunYing SUN, XiaoYe ZHANG, WeiJun LI, Factors contributing to haze and fog in China Chinese Science Bulletin. ,vol. 58, pp. 1178- 1187 ,(2013) , 10.1360/972013-150
Gehui Wang, Renyi Zhang, Mario E. Gomez, Lingxiao Yang, Misti Levy Zamora, Min Hu, Yun Lin, Jianfei Peng, Song Guo, Jingjing Meng, Jianjun Li, Chunlei Cheng, Tafeng Hu, Yanqin Ren, Yuesi Wang, Jian Gao, Junji Cao, Zhisheng An, Weijian Zhou, Guohui Li, Jiayuan Wang, Pengfei Tian, Wilmarie Marrero-Ortiz, Jeremiah Secrest, Zhuofei Du, Jing Zheng, Dongjie Shang, Limin Zeng, Min Shao, Weigang Wang, Yao Huang, Yuan Wang, Yujiao Zhu, Yixin Li, Jiaxi Hu, Bowen Pan, Li Cai, Yuting Cheng, Yuemeng Ji, Fang Zhang, Daniel Rosenfeld, Peter S. Liss, Robert A. Duce, Charles E. Kolb, Mario J. Molina, Persistent sulfate formation from London Fog to Chinese haze Proceedings of the National Academy of Sciences of the United States of America. ,vol. 113, pp. 13630- 13635 ,(2016) , 10.1073/PNAS.1616540113