Hybrid LES–multizonal modelling of the uranium oxalate precipitation

作者: M. Bertrand , E. Plasari , O. Lebaigue , P. Baron , N. Lamarque

DOI: 10.1016/J.CES.2012.03.019

关键词:

摘要: Abstract Oxalic precipitation is usually applied to process radioactive wastes or recover actinides from a multicomponent solution. Due their later handling and use, actinide precipitates have satisfy strict requirements. In nuclear environment where experiments are limited, simulation may be the only way test different industrial configurations in order adjust campaigns. this manuscript, modelling of tetravalent uranium oxalate an unbaffled reactor achieved using hybrid multizonal/CFD model. The population balance solved according moment method multizonal model entirely parameterised through computational fluid dynamics calculations based on large-eddy (LES) sub-grid micromixing. show how specificity flow field can noticeable effect properties.

参考文章(32)
F. Bezzo, S. Macchietto, C.C. Pantelides, A general methodology for hybrid multizonal/CFD models Computers & Chemical Engineering. ,vol. 28, pp. 501- 511 ,(2004) , 10.1016/J.COMPCHEMENG.2003.08.004
C. Calvin, Ph. Emonot, The TRIO-Unitaire Project: A Parallel CFD 3-Dimensional Code conference on scientific computing. pp. 169- 176 ,(1997) , 10.1007/3-540-63827-X_58
F. Nicoud, F. Ducros, Subgrid-scale stress modelling based on the square of the velocity gradient tensor Flow Turbulence and Combustion. ,vol. 62, pp. 183- 200 ,(1999) , 10.1023/A:1009995426001
The Growth of Crystals and the Equilibrium Structure of their Surfaces Philosophical transactions - Royal Society. Mathematical, physical and engineering sciences. ,vol. 243, pp. 299- 358 ,(1951) , 10.1098/RSTA.1951.0006
Tariq Mahmud, Jennifer N. Haque, Kevin J. Roberts, Dominic Rhodes, Derek Wilkinson, Measurements and modelling of free-surface turbulent flows induced by a magnetic stirrer in an unbaffled stirred tank reactor Chemical Engineering Science. ,vol. 64, pp. 4197- 4209 ,(2009) , 10.1016/J.CES.2009.06.059
C. Jiménez, F. Ducros, B. Cuenot, B. Bédat, Subgrid scale variance and dissipation of a scalar field in large eddy simulations Physics of Fluids. ,vol. 13, pp. 1748- 1754 ,(2001) , 10.1063/1.1366668
Hyun Sik Yoon, S. Balachandar, Man Yeong Ha, Large eddy simulation of flow in an unbaffled stirred tank for different Reynolds numbers Physics of Fluids. ,vol. 21, pp. 085102- ,(2009) , 10.1063/1.3210776
Lian-Ping Wang, Anthony S. Wexler, Yong Zhou, On the collision rate of small particles in isotropic turbulence. II. Finite inertia case Physics of Fluids. ,vol. 10, pp. 1206- 1216 ,(1998) , 10.1063/1.869565
A.A. Öncül, K. Sundmacher, A. Seidel-Morgenstern, D. Thévenin, Numerical and analytical investigation of barium sulphate crystallization Chemical Engineering Science. ,vol. 61, pp. 652- 664 ,(2006) , 10.1016/J.CES.2005.07.037
Alessandro Zucca, Daniele L. Marchisio, Antonello A. Barresi, Rodney O. Fox, Implementation of the population balance equation in CFD codes for modelling soot formation in turbulent flames Chemical Engineering Science. ,vol. 61, pp. 87- 95 ,(2006) , 10.1016/J.CES.2004.11.061