Nanometer-sized particle formation from NH3/SO2/H2O/Air mixtures by ionizing irradiation
作者： Tae Oh Kim , Takashi Ishida , Motoaki Adachi , Kikuo Okuyama , John H. Seinfeld
DOI: 10.1080/02786829808965556
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摘要: ABSTRACT Formation of nanometer-sized particles in NH3/SO2/H2O/Air mixtures by α-ray irradiation was studied experimentally to evaluate the effect NH3 gas on gas-to-particle conversion process. The total particle number concentration, charged-particle fraction, and electrical mobility distribution generated ionization chamber were measured at various NH3, SO2, H2O vapor concentrations residence times mixture. Particle generation enhanced presence but enhancement depends greatly concentrations; mixing ratios 0.71–3.6 ppm 2–4 higher than those absence constant this range concentration. fraction decreased with addition which indicated that ion-induced nucleation homogeneous enhanced. To gaseous products, kinetic equations...
sci-hub.se 参考文章(44)
Gaunlin Shen, Masako Suto, L. C. Lee, Reaction rate constant of SO3+ NH3in the gas phase Journal of Geophysical Research. ,vol. 95, pp. 13981- 13984 ,(1990) , 10.1029/JD095ID09P13981
B. Kärcher, Th. Peter, R. Ottmann, Contrail formation: Homogeneous nucleation of H2SO4/H2O droplets Geophysical Research Letters. ,vol. 22, pp. 1501- 1504 ,(1995) , 10.1029/95GL01337
Antomy D. Clarke, ATMOSPHERIC NUCLEI IN THE REMOTE FREE-TROPOSPHERE Journal of Atmospheric Chemistry. ,vol. 14, pp. 479- 488 ,(1992) , 10.1007/BF00115252
W.D. Scott, F.C.R. Cattell, Vapor pressure of ammonium sulfates Atmospheric Environment (1967). ,vol. 13, pp. 307- 317 ,(1979) , 10.1016/0004-6981(79)90174-4
Moo Been Chang, Mark J Kushner, Mark J Rood, None, Removal of SO2 and the simultaneous removal of SO2 and NO from simulated flue gas streams using dielectric barrier discharge plasmas Plasma Chemistry and Plasma Processing. ,vol. 12, pp. 565- 580 ,(1992) , 10.1007/BF01447259
M. Neugebauer, B. Buti, A search for evidence of the evolution of rotational discontinuities in the solar wind from nonlinear Alfvén waves Journal of Geophysical Research. ,vol. 95, pp. 13- 20 ,(1990) , 10.1029/JA095IA01P00013
Takafumi Seto, Tatsuya Nakamoto, Kikuo Okuyama, Motoaki Adachi, Yoshikazu Kuga, Kazuo Takeuchi, Size distribution measurement of nanometer-sized aerosol particles using dma under low-pressure conditions Journal of Aerosol Science. ,vol. 28, pp. 193- 206 ,(1997) , 10.1016/S0021-8502(96)00071-7
F. Raes, A. Janssens, G. Eggermont, A synergism between ultraviolet and gamma radiation in producing aerosol particles from SO2H2SO4 laden atmospheres Atmospheric Environment. ,vol. 19, pp. 1069- 1073 ,(1985) , 10.1016/0004-6981(85)90191-X
Peter Seier Christensen, Stig Wedel, Hans Livbjerg, The kinetics of the photolytic production of aerosols from SO2 and NH3 in humid air Chemical Engineering Science. ,vol. 49, pp. 4605- 4614 ,(1994) , 10.1016/S0009-2509(05)80044-2
R. C. Brown, R. C. Miake-Lye, M. R. Anderson, C. E. Kolb, T. J. Resch, Aerosol dynamics in near-field aircraft plumes Journal of Geophysical Research: Atmospheres. ,vol. 101, pp. 22939- 22953 ,(1996) , 10.1029/96JD01918