Molecular Vibrations in Liquids: Direct Measurement of the Molecular Dephasing Time; Determination of the Shape of Picosecond Light Pulses

作者: D. von der Linde , A. Laubereau , W. Kaiser

DOI: 10.1103/PHYSREVLETT.26.954

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摘要: Molecular vibrations are coherently excited by an intense light pulse of duration ${t}_{p}$. The rise and decay the vibrational amplitude is measured with delayed pulses same time dependence. molecular dephasing $\ensuremath{\tau}$ obtained when $\ensuremath{\tau}\ensuremath{\gtrsim}{t}_{p}$, while shape found for $\ensuremath{\tau}\ensuremath{\ll}{t}_{p}$.

参考文章(10)
J. A. Giordmaine, W. Kaiser, Light Scattering by Coherently Driven Lattice Vibrations Physical Review. ,vol. 144, pp. 676- 688 ,(1966) , 10.1103/PHYSREV.144.676
A. K. McQuillan, W. R. L. Clements, B. P. Stoicheff, Stimulated Raman Emission in Diamond: Spectrum, Gain, and Angular Distribution of Intensity Physical Review A. ,vol. 1, pp. 628- 635 ,(1970) , 10.1103/PHYSREVA.1.628
F. DeMartini, J. Ducuing, Stimulated Raman Scattering in Hydrogen: A Measurement of the Vibrational Lifetime Physical Review Letters. ,vol. 17, pp. 117- 119 ,(1966) , 10.1103/PHYSREVLETT.17.117
D. von der Linde, M. Maier, W. Kaiser, Quantitative Investigations of the Stimulated Raman Effect Using Subnanosecond Light Pulses Physical Review. ,vol. 178, pp. 11- 17 ,(1969) , 10.1103/PHYSREV.178.11
M. Maier, W. Kaiser, J. A. Giordmaine, Backward Stimulated Raman Scattering Physical Review. ,vol. 177, pp. 580- 599 ,(1969) , 10.1103/PHYSREV.177.580
S.A. Akhmanov, Transient effects in stimulated Raman scattering Materials Research Bulletin. ,vol. 4, pp. 455- 462 ,(1969) , 10.1016/0025-5408(69)90104-4
R. L. Carman, F. Shimizu, C. S. Wang, N. Bloembergen, Theory of Stokes Pulse Shapes in Transient Stimulated Raman Scattering Physical Review A. ,vol. 2, pp. 60- 72 ,(1970) , 10.1103/PHYSREVA.2.60
D. von der Linde, O. Bernecker, A. Laubereau, A fast electrooptic shutter for the selection of single picosecond laser pulses Optics Communications. ,vol. 2, pp. 215- 218 ,(1970) , 10.1016/0030-4018(70)90141-0
D. Von Der Linde, O. Bernecker, W. Kaiser, Experimental investigation of single picosecond pulses Optics Communications. ,vol. 2, pp. 149- 152 ,(1970) , 10.1016/0030-4018(70)90001-5
J. A. Giordmaine, P. M. Rentzepis, S. L. Shapiro, K. W. Wecht, TWO‐PHOTON EXCITATION OF FLUORESCENCE BY PICOSECOND LIGHT PULSES Applied Physics Letters. ,vol. 11, pp. 216- 218 ,(1967) , 10.1063/1.1755105