Characterization and source identification of airborne trace metals in Singapore.

作者: R. Balasubramanian , W-B. Qian

DOI: 10.1039/B407523D

关键词:

摘要: Airborne particulate trace metals have important health implications. As a consequence, their concentrations are increasingly monitored in many urban locations worldwide. In this study, fine atmospheric particles (PM2.5) were collected Singapore over period of 83 consecutive days during 2000, and analysed to determine the concentration elements using ICP-MS. Altogether, eighteen airborne quantified: Al, Ag, Ba, Cd, Cr, Co, Cu, Fe, Ga, Li, Mn, Ni, Pb, Sr, Zn, V, Si, Ti. While Li was least abundant metal with mean 0.2 ng m−3, Zn showed maximum 279.1 m−3. Calculation enrichment factors indicated that Cu enriched by 30 5000 relative natural abundance crustal soil. The extent pollution study area assessed comparing measured those reported literature for selected number sites other parts world. Factor analysis used identify major sources affecting air Singapore. contribute loading metal-bearing aerosols atmosphere include fuel oil-fired power plants, processing industry, land reclamation construction activities, municipal solid waste incinerators, traffic emissions.

参考文章(16)
Y.C. Chan, R.W. Simpson, G.H. McTainsh, P.D. Vowles, D.D. Cohen, G.M. Bailey, Characterisation of chemical species in PM2.5 and PM10 aerosols in Brisbane, Australia Atmospheric Environment. ,vol. 31, pp. 3773- 3785 ,(1997) , 10.1016/S1352-2310(97)00213-6
R. Chester, M. Nimmo, G.R. Fones, S. Keyse, Z. Zhang, Trace metal chemistry of particulate aerosols from the UK mainland coastal rim of the NE Irish sea. Atmospheric Environment. ,vol. 34, pp. 949- 958 ,(2000) , 10.1016/S1352-2310(99)00234-4
R. Balasubramanian, T. Victor, R. Begum, Impact of biomass burning on rainwater acidity and composition in Singapore Journal of Geophysical Research: Atmospheres. ,vol. 104, pp. 26881- 26890 ,(1999) , 10.1029/1999JD900247
Mustafa Yatin, Semra Tuncel, Namik K. Aras, Ilhan Olmez, Sezer Aygun, Gurdal Tuncel, Atmospheric trace elements in Ankara, Turkey: 1. factors affecting chemical composition of fine particles Atmospheric Environment. ,vol. 34, pp. 1305- 1318 ,(2000) , 10.1016/S1352-2310(98)00297-0
J F Gamble, R J Lewis, Health and respirable particulate (PM10) air pollution: a causal or statistical association? Environmental Health Perspectives. ,vol. 104, pp. 838- 850 ,(1996) , 10.1289/EHP.96104838
C. Arden Pope, Joel Schwartz, Michael R. Ransom, Daily mortality and PM10 pollution in Utah Valley. Archives of Environmental Health. ,vol. 47, pp. 211- 217 ,(1992) , 10.1080/00039896.1992.9938351
Judith C. Chow, John G. Watson, Eric M. Fujita, Zhiqiang Lu, Douglas R. Lawson, Lowell L. Ashbaugh, Temporal and spatial variations of PM2.5 and PM10 aerosol in the Southern California air quality study Atmospheric Environment. ,vol. 28, pp. 2061- 2080 ,(1994) , 10.1016/1352-2310(94)90474-X
Guor-Cheng Fang, Cheng-Nan Chang, Yuh-Shen Wu, Peter Pi-Cheng Fu, Ding-Guor Yang, Chu Chia-Chium, Characterization of chemical species in PM2.5 and PM10 aerosols in suburban and rural sites of central Taiwan. Science of The Total Environment. ,vol. 234, pp. 203- 212 ,(1999) , 10.1016/S0048-9697(99)00276-4
Javier Miranda, Thomas A. Cahill, J.Roberto Morales, F. Aldape, J.M. Flores, R.V. Díaz, Determination of elemental concentrations in atmospheric aerosols in mexico city using proton induced x-ray emission, proton elastic scattering, and laser absorption Atmospheric Environment. ,vol. 28, pp. 2299- 2306 ,(1994) , 10.1016/1352-2310(94)90483-9