Enhancing Photocatalytic Activity on (MnO@TNTAs):Mn 2+ with a Hierarchical Sandwich-Like Nanostructure via a Two-Step Procedure

作者: Junhan Kong , Wei Zhang , Yubo Zhang , Minghao Xia , Xiuling Wu

DOI: 10.1007/S11664-018-6148-2

关键词:

摘要: Several semiconductor nanomaterial devices are increasingly being applied in a variety of fields, especially the treating environmental pollutants. We have fabricated (MnO@TNTAs):Mn2+ with sandwich-like nanostructures composed TiO2 nanotube arrays (TNTAs), Mn-doped TNTAs and MnO. The experimental procedure was two-step synthesis: first, using anodic oxidation methods then hydrothermal methods. carried out many characterizations “sandwiches“ nanoscale. From field emission scanning electron microscopy images we found nanofibers lying on highly-ordered arrays. diameter nanotubes about 50 nm but size varied. Energy dispersive spectroscopy demonstrated that contained manganese element x-ray diffraction patterns showed peak manganosite phase. ultraviolet–visible light spectra, it had strong absorption activities under both ultraviolet visible radiation, while pure only light. photodegradation experiments proved an excellent photocatalytic activity (92.5% after 240 min), which great improvement compared TNTAs. In this way, structures as device at nanoscale huge potential controlling pollution.

参考文章(20)
Alagesan Subramanian, Hong-Wen Wang, Effects of boron doping in TiO2 nanotubes and the performance of dye-sensitized solar cells Applied Surface Science. ,vol. 258, pp. 6479- 6484 ,(2012) , 10.1016/J.APSUSC.2012.03.064
Xiaoxiao Li, Yuejun Zhang, Xiaolei Zhao, Nana Gao, Tao Fu, The characteristics of sludge from enhanced coagulation processes using PAC/PDMDAAC composite coagulants in treatment of micro-polluted raw water Separation and Purification Technology. ,vol. 147, pp. 125- 131 ,(2015) , 10.1016/J.SEPPUR.2015.04.015
Yongpeng Xu, Ting Chen, Fuyi Cui, Wenxin Shi, Effect of reused alum-humic-flocs on coagulation performance and floc characteristics formed by aluminum salt coagulants in humic-acid water Chemical Engineering Journal. ,vol. 287, pp. 225- 232 ,(2016) , 10.1016/J.CEJ.2015.11.017
Eseoghene H. Umukoro, Moses G. Peleyeju, Jane C. Ngila, Omotayo A. Arotiba, Photocatalytic degradation of acid blue 74 in water using Ag–Ag2O–Zno nanostuctures anchored on graphene oxide Solid State Sciences. ,vol. 51, pp. 66- 73 ,(2016) , 10.1016/J.SOLIDSTATESCIENCES.2015.11.015
E. Dumont, A. Couvert, A. Amrane, C. Couriol, G. Darracq, P. Le Cloirec, Equivalent Absorption Capacity (EAC) concept applied to the absorption of hydrophobic VOCs in a water/PDMS mixture Chemical Engineering Journal. ,vol. 287, pp. 205- 216 ,(2016) , 10.1016/J.CEJ.2015.11.020
Alireza Allafchian, Seyed Amir Hossein Jalali, Hamid Bahramian, Hossein Ahmadvand, Preparation, characterization, and antibacterial activity of NiFe2O4/PAMA/Ag–TiO2 nanocomposite Journal of Magnetism and Magnetic Materials. ,vol. 404, pp. 14- 20 ,(2016) , 10.1016/J.JMMM.2015.12.015
S.A. Ahmed, Annealing effects on structure and magnetic properties of Mn-doped TiO2 Journal of Magnetism and Magnetic Materials. ,vol. 402, pp. 178- 183 ,(2016) , 10.1016/J.JMMM.2015.11.065
Krishnamoorthy Krishnadevi, Vaithilingam Selvaraj, Cyclotriphosphazene and TiO2 reinforced nanocomposite coated on mild steel plates for antibacterial and corrosion resistance applications Applied Surface Science. ,vol. 366, pp. 148- 157 ,(2016) , 10.1016/J.APSUSC.2016.01.018
Lingfan Zhang, Tianyi Zhu, Xin Liu, Wenqing Zhang, Simultaneous oxidation and adsorption of As(III) from water by cerium modified chitosan ultrafine nanobiosorbent. Journal of Hazardous Materials. ,vol. 308, pp. 1- 10 ,(2016) , 10.1016/J.JHAZMAT.2016.01.015
Diana Mardare, Nicoleta Cornei, Carmen Mita, Daniel Florea, Alexandru Stancu, Vasile Tiron, Alina Manole, Catalin Adomnitei, Low temperature TiO2 based gas sensors for CO2 Ceramics International. ,vol. 42, pp. 7353- 7359 ,(2016) , 10.1016/J.CERAMINT.2016.01.137