Increase in background stratospheric aerosol observed with lidar at Mauna Loa Observatory and Boulder, Colorado

作者: David Hofmann , John Barnes , Michael O'Neill , Michael Trudeau , Ryan Neely

DOI: 10.1029/2009GL039008

关键词:

摘要: [1] The stratospheric aerosol layer has been monitored with lidars at Mauna Loa Observatory in Hawaii and Boulder Colorado since 1975 2000, respectively. Following the Pinatubo volcanic eruption June 1991, global stratosphere not perturbed by a major providing an unprecedented opportunity to study background aerosol. Since about increase of 4–7% per year backscatter altitude range 20–30 km detected both Boulder. This is superimposed on seasonal cycle winter maximum that modulated quasi-biennial oscillation (QBO) tropical winds. Of three causes for increase: emissions stratosphere, increased upwelling, anthropogenic sulfur gas troposphere, it appears large coal burning 2002, mainly China, likely source dioxide ultimately ends up as sulfate responsible from layer. The results are consistent 0.6–0.8% tropospheric entering stratosphere.

参考文章(18)
R. J. CHARLSON, S. E. SCHWARTZ, J. M. HALES, R. D. CESS, J. A. COAKLEY, J. E. HANSEN, D. J. HOFMANN, Climate Forcing by Anthropogenic Aerosols Science. ,vol. 255, pp. 423- 430 ,(1992) , 10.1126/SCIENCE.255.5043.423
Erik Kjellström, A Three-Dimensional Global Model Study of Carbonyl Sulfide in the Troposphere and the Lower Stratosphere Journal of Atmospheric Chemistry. ,vol. 29, pp. 151- 177 ,(1998) , 10.1023/A:1005976511096
Jonathan H. Jiang, Bin Wang, Kenshi Goya, Klemens Hocke, Stephen D. Eckermann, Jun Ma, Dong L. Wu, William G. Read, Geographical distribution and interseasonal variability of tropical deep convection: UARS MLS observations and analyses Journal of Geophysical Research: Atmospheres. ,vol. 109, pp. n/a- n/a ,(2004) , 10.1029/2003JD003756
S. A. Montzka, P. Calvert, B. D. Hall, J. W. Elkins, T. J. Conway, P. P. Tans, C. Sweeney, On the global distribution, seasonality, and budget of atmospheric carbonyl sulfide (COS) and some similarities to CO2 Journal of Geophysical Research. ,vol. 112, ,(2007) , 10.1029/2006JD007665
David J. Hofmann, Susan Solomon, Ozone destruction through heterogeneous chemistry following the eruption of El Chichón Journal of Geophysical Research. ,vol. 94, pp. 5029- 5041 ,(1989) , 10.1029/JD094ID04P05029
J. E. Barnes, D. J. Hofmann, Variability in the stratospheric background aerosol over Mauna Loa Observatory Geophysical Research Letters. ,vol. 28, pp. 2895- 2898 ,(2001) , 10.1029/2001GL013127
Steven J Smith, Hugh Pitcher, T.M.L Wigley, Global and regional anthropogenic sulfur dioxide emissions grid and pervasive computing. ,vol. 29, pp. 99- 119 ,(2001) , 10.1016/S0921-8181(00)00057-6
William J. Randel, Fei Wu, Holger Vömel, Gerald E. Nedoluha, Piers Forster, Decreases in stratospheric water vapor after 2001: Links to changes in the tropical tropopause and the Brewer-Dobson circulation Journal of Geophysical Research. ,vol. 111, ,(2006) , 10.1029/2005JD006744
Kirk W. Thoning, Pieter P. Tans, Walter D. Komhyr, Atmospheric carbon dioxide at Mauna Loa Observatory: 2. Analysis of the NOAA GMCC data, 1974-1985 Journal of Geophysical Research: Atmospheres. ,vol. 94, pp. 8549- 8565 ,(1989) , 10.1029/JD094ID06P08549
D. J. HOFMANN, Aircraft sulphur emissions Nature. ,vol. 349, pp. 659- 659 ,(1991) , 10.1038/349659A0