Vibrational predissociation dynamics of the nitric oxide dimer

摘要: We have studied the photofragmentation of NO dimer employing quasi-classical trajectories propagation using quantum probabilities distributions and Wigner distribution functions to determine initial conditions system. The in phase space, between distributions, are not so different. depends strongly on excitation state, especially for lowest them. These results concordance with experimental values where we can see a similar tendency lifetimes different vibrational modes that been studied. In this work explore more intramolecular intermolecular modes. increased number dissociation distance simulation as well.