Rydberg-state ionization dynamics and tunnel ionization rates in strong electric fields

作者: K. Gawlas , S. D. Hogan

DOI: 10.1103/PHYSREVA.99.013421

关键词:

摘要: Tunnel ionization rates of triplet Rydberg states in helium with principal quantum numbers close to 37 have been measured electric fields at the classical threshold $\ensuremath{\sim}197$ V/cm. The measurements were performed time domain by combining high-resolution continuous-wave laser photoexcitation and pulsed field ionization. observed tunnel range from ${10}^{5}$ ${10}^{7}\phantom{\rule{4pt}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}$ have, together atomic energy-level structure corresponding fields, compared results calculations eigenvalues Hamiltonian matrix describing atoms presence which complex absorbing potentials introduced. comparison these, additional for hydrogenlike using semiempirical methods, allowed accuracy these methods calculation be tested. For particular eigenstates studied are $\ensuremath{\sim}5$ times larger than those obtained expressions.

参考文章(32)
F. B. Dunning, R. F. Stebbings, Rydberg States of Atoms and Molecules ,(2011)
J. A. Gibbard, M. Dethlefsen, M. Kohlhoff, C. J. Rennick, E. So, M. Ford, T. P. Softley, Resonant Charge Transfer of Hydrogen Rydberg Atoms Incident on a Cu(100) Projected Band-Gap Surface Physical Review Letters. ,vol. 115, pp. 093201- 093201 ,(2015) , 10.1103/PHYSREVLETT.115.093201
F. G. Kellert, K. A. Smith, R. D. Rundel, F. B. Dunning, R. F. Stebbings, Collisions of xenon (nf) Rydberg atoms with ammonia The Journal of Chemical Physics. ,vol. 72, pp. 3179- 3190 ,(1980) , 10.1063/1.439551
T Halfmann, J Koensgen, K Bergmann, A source for a high-intensity pulsed beam of metastable helium atoms Measurement Science and Technology. ,vol. 11, pp. 1510- 1514 ,(2000) , 10.1088/0957-0233/11/10/312
Non-Adiabatic Crossing of Energy Levels Proceedings of The Royal Society A: Mathematical, Physical and Engineering Sciences. ,vol. 137, pp. 696- 702 ,(1932) , 10.1098/RSPA.1932.0165
G. R. Lloyd, S. R. Procter, T. P. Softley, Ionization of hydrogen Rydberg molecules at a metal surface. Physical Review Letters. ,vol. 95, pp. 133202- ,(2005) , 10.1103/PHYSREVLETT.95.133202
A. Osterwalder, F. Merkt, Using High Rydberg States as Electric Field Sensors Physical Review Letters. ,vol. 82, pp. 1831- 1834 ,(1999) , 10.1103/PHYSREVLETT.82.1831
E. H. Hauge, J. A. Støvneng, Tunneling times: a critical review Reviews of Modern Physics. ,vol. 61, pp. 917- 936 ,(1989) , 10.1103/REVMODPHYS.61.917
Willem van de Water, David R. Mariani, Peter M. Koch, Ionization of highly excited helium atoms in an electric field Physical Review A. ,vol. 30, pp. 2399- 2412 ,(1984) , 10.1103/PHYSREVA.30.2399
S. B. Hill, C. B. Haich, Z. Zhou, P. Nordlander, F. B. Dunning, Ionization of xenon Rydberg atoms at a metal surface. Physical Review Letters. ,vol. 85, pp. 5444- 5447 ,(2000) , 10.1103/PHYSREVLETT.85.5444